RNA m5C oxidation by TET2 regulates chromatin state and leukaemogenesis

Nature. 2024 Oct;634(8035):986-994. doi: 10.1038/s41586-024-07969-x. Epub 2024 Oct 2.

Abstract

Mutation of tet methylcytosine dioxygenase 2 (encoded by TET2) drives myeloid malignancy initiation and progression1-3. TET2 deficiency is known to cause a globally opened chromatin state and activation of genes contributing to aberrant haematopoietic stem cell self-renewal4,5. However, the open chromatin observed in TET2-deficient mouse embryonic stem cells, leukaemic cells and haematopoietic stem and progenitor cells5 is inconsistent with the designated role of DNA 5-methylcytosine oxidation of TET2. Here we show that chromatin-associated retrotransposon RNA 5-methylcytosine (m5C) can be recognized by the methyl-CpG-binding-domain protein MBD6, which guides deubiquitination of nearby monoubiquitinated Lys119 of histone H2A (H2AK119ub) to promote an open chromatin state. TET2 oxidizes m5C and antagonizes this MBD6-dependent H2AK119ub deubiquitination. TET2 depletion thereby leads to globally decreased H2AK119ub, more open chromatin and increased transcription in stem cells. TET2-mutant human leukaemia becomes dependent on this gene activation pathway, with MBD6 depletion selectively blocking proliferation of TET2-mutant leukaemic cells and largely reversing the haematopoiesis defects caused by Tet2 loss in mouse models. Together, our findings reveal a chromatin regulation pathway by TET2 through retrotransposon RNA m5C oxidation and identify the downstream MBD6 protein as a feasible target for developing therapies specific against TET2 mutant malignancies.

MeSH terms

  • 5-Methylcytosine* / metabolism
  • Animals
  • Carcinogenesis* / genetics
  • Carcinogenesis* / metabolism
  • Carcinogenesis* / pathology
  • Cell Proliferation
  • Cell Self Renewal
  • Chromatin* / chemistry
  • Chromatin* / genetics
  • Chromatin* / metabolism
  • DNA-Binding Proteins* / deficiency
  • DNA-Binding Proteins* / genetics
  • DNA-Binding Proteins* / metabolism
  • Dioxygenases* / deficiency
  • Dioxygenases* / genetics
  • Dioxygenases* / metabolism
  • Female
  • Hematopoiesis
  • Histones / chemistry
  • Histones / metabolism
  • Humans
  • Leukemia* / genetics
  • Leukemia* / metabolism
  • Leukemia* / pathology
  • Male
  • Mice
  • Mutation
  • Oxidation-Reduction
  • RNA* / chemistry
  • RNA* / genetics
  • RNA* / metabolism
  • Retroelements / genetics
  • Transcription, Genetic
  • Ubiquitination

Substances

  • 5-Methylcytosine
  • Chromatin
  • Dioxygenases
  • DNA-Binding Proteins
  • Histones
  • MBD6 protein, human
  • Retroelements
  • RNA
  • TET2 protein, human
  • Tet2 protein, mouse