Selective and asymmetric action of trypsin on the dimeric forms of seminal RNase

Protein Sci. 1998 Dec;7(12):2653-8. doi: 10.1002/pro.5560071219.

Abstract

Dimeric seminal RNase (BS-RNase) is an equilibrium mixture of conformationally different quaternary structures, one characterized by the interchange between subunits of their N-terminal ends (the MXM form); the other with no interchange (the M=M form). Controlled tryptic digestion of each isolated quaternary form generates, as limit digest products, folded and enzymatically active molecules, very resistant to further tryptic degradation. Electrospray mass spectrometric analyses and N-terminal sequence determinations indicate that trypsin can discriminate between the conformationally different quaternary structures of seminal RNase, and exerts a differential and asymmetric action on the two dimeric forms, depending on the original quaternary conformation of each form. The two digestion products from the MXM and the M=M dimeric forms have different structures, which are reminiscent of the original quaternary conformation of the dimers: one with interchange, the other with no interchange, of the N-terminal ends. The surprising resistance of these tryptic products to further tryptic action is explained by the persistence in each digestion product of the original intersubunit interface.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cattle
  • Dimerization
  • Hydrolysis
  • Male
  • Mass Spectrometry / methods
  • Models, Molecular
  • Peptide Fragments / chemistry
  • Peptide Fragments / metabolism
  • Protein Conformation
  • Ribonucleases / chemistry*
  • Ribonucleases / isolation & purification
  • Ribonucleases / metabolism*
  • Semen / enzymology*
  • Trypsin / chemistry
  • Trypsin / metabolism*

Substances

  • Peptide Fragments
  • Ribonucleases
  • Trypsin