Structure and function of microplasminogen: I. Methionine shuffling, chemical proteolysis, and proenzyme activation

Protein Sci. 1995 Sep;4(9):1758-67. doi: 10.1002/pro.5560040911.

Abstract

We have cloned and expressed microplasminogen (mPlg), consisting of the N-terminal undecapeptide of human glu-Plg spliced to its proenzyme domain. This truncated (approximately 28 kDa) proenzyme retained the distinctive catalytic activities of the larger parent. Replacement of M residues followed by M shuffling permitted subsequent scission by site-directed chemical proteolysis (in CNBr/formic acid) without impairing any of the protein's characteristic properties. Activation of chymotrypsinogen-related zymogens occurs by limited proteolysis; the newly liberated, highly conserved N-terminus (VVGG) forms a salt bridge with an aspartyl residue immediately upstream of the active site serine. The role of both of these elements in mPlg activation was probed using protein engineering and site-directed proteolysis to alter the length and amino acid composition of the N-terminus, and to replace the aspartate. All modifications affected both Km and Kcat. The results identify some structural parameters of the N-terminus required for proenzyme activation.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Base Sequence
  • Cloning, Molecular
  • Cyanogen Bromide / chemistry*
  • Enzyme Activation
  • Enzyme Precursors / chemistry*
  • Enzyme Precursors / metabolism
  • Escherichia coli / genetics
  • Formates / chemistry*
  • Humans
  • Methionine / chemistry*
  • Molecular Sequence Data
  • Mutagenesis
  • Plasminogen / chemistry*
  • Plasminogen / genetics
  • Plasminogen / metabolism
  • Protein Engineering
  • Recombinant Proteins
  • Restriction Mapping

Substances

  • Enzyme Precursors
  • Formates
  • Recombinant Proteins
  • formic acid
  • Plasminogen
  • Methionine
  • Cyanogen Bromide