Rg3-lipo biomimetic delivery of paclitaxel enhances targeting of tumors and myeloid-derived suppressor cells

J Clin Invest. 2024 Nov 15;134(22):e178617. doi: 10.1172/JCI178617.

Abstract

Liposomal drug delivery systems have revolutionized traditional cytotoxic drugs. However, the relative instability and toxicity of the existing liposomal drug delivery systems compromised their efficacy. Herein, we present Rg3-lipo, an innovative drug delivery system using a glycosyl moiety-enriched ginsenoside (Rg3). This system is distinguished by its glycosyl moieties exposed on the liposomal surface. These moieties imitate human cell membranes to stabilize and evade phagocytic clearance. The Rg3-lipo system loaded with paclitaxel (PTX-Rg3-lipo) demonstrated favorable bioavailability and safety in Sprague-Dawley rats, beagle dogs, and cynomolgus monkeys. With its glycosyl moieties recognizing tumor cells via the glucose transporter Glut1, PTX-Rg3-lipo inhibited gastric, breast, and esophageal cancers in human cancer cell lines, tumor-bearing mice, and patient-derived xenograft models. These glycosyl moieties selectively targeted myeloid-derived suppressor cells (MDSCs) through the glucose transporter Glut3 to attenuate their immunosuppressive effect. The mechanism study revealed that Rg3-lipo suppressed glycolysis and downregulated the transcription factors c-Maf and Mafb overcoming the MDSC-mediated immunosuppressive microenvironment and enhancing PTX-Rg3-lipo's antitumor effect. Taken together, we supply substantial evidence for its advantageous bioavailability and safety in multiple animal models, including nonhuman primates, and Rg3-lipo's dual targeting of cancer cells and MDSCs. Further investigation regarding Rg3-lipo's druggability will be conducted in clinical trials.

Keywords: Drug therapy; Immunology; Immunotherapy; Therapeutics.

MeSH terms

  • Animals
  • Antineoplastic Agents, Phytogenic / chemistry
  • Antineoplastic Agents, Phytogenic / pharmacology
  • Cell Line, Tumor
  • Dogs
  • Drug Delivery Systems
  • Female
  • Ginsenosides* / chemistry
  • Ginsenosides* / pharmacokinetics
  • Ginsenosides* / pharmacology
  • Humans
  • Liposomes / chemistry
  • Macaca fascicularis*
  • Male
  • Mice
  • Myeloid-Derived Suppressor Cells* / drug effects
  • Myeloid-Derived Suppressor Cells* / metabolism
  • Neoplasms / drug therapy
  • Neoplasms / metabolism
  • Neoplasms / pathology
  • Paclitaxel* / chemistry
  • Paclitaxel* / pharmacology
  • Rats
  • Rats, Sprague-Dawley
  • Xenograft Model Antitumor Assays

Substances

  • Paclitaxel
  • Ginsenosides
  • Liposomes
  • ginsenoside Rg3
  • Antineoplastic Agents, Phytogenic