Characterization of experimental resin composites with cholesteryl methacrylate organic matrix - Part 2

Dent Mater. 2024 Nov;40(11):e63-e71. doi: 10.1016/j.dental.2024.07.037. Epub 2024 Aug 7.

Abstract

Objective: The aim of this study was to evaluate the degree of conversion (%), flexural strength (MPa), elastic modulus (GPa), compressive strength (MPa), Knoop microhardness (KHN), post-gel shrinkage (%) and prediction of ideal concentration of cholesteryl methacrylate (CM) in experimental resins.

Methods: Four formulations were manipulated (F): F1, control group, (0 % CM); F2 (15 % CM); F3 (19.8 % CM) and F4 (30 % CM). Bis-GMA and CM percentages were determined using Statistica™ software. For the degree of conversion test, Raman spectroscopy was used. To testing flexural strength, elastic modulus and compressive strength, a universal testing machine was used. For the Knoop microhardness test five indentations were made in each sample. Post-gel shrinkage was determined using the strain gauge method. Statistica™ software processed all data obtained in this study. Results were submitted to one-way ANOVA and Tukey's post hoc tests (α = 0.05).

Results: Better performance was observed for F2 (15 % CM) and F3 (19,8 % CM) for degree of conversion, elastic modulus and post-gel shrinkage. For Knoop microhardness F2 (15 % CM), F3 (19,8 % CM) and F4 (30 % CM) showed higher values than F1 (0 % CM). For flexural strength F1 (0 % CM) and F3 (19,8 %) were similar and F4 showed the lowest values and for compressive strength F1 (0 % CM) showed the highest values. For mixture designs analysis data, concentrations ≤ 25 % of CM would provide better results.

Significance: Addition of CM at concentrations lower than 30 % contributed to a significant increase in the degree of conversion, microhardness values, elastic modulus and reduction of post-gel shrinkage.

Keywords: Cholesterol Esters; Composite Resins; Methacrylates; Polymerization; Polymers.

MeSH terms

  • Bisphenol A-Glycidyl Methacrylate / chemistry
  • Composite Resins* / chemistry
  • Compressive Strength*
  • Dental Stress Analysis
  • Elastic Modulus*
  • Flexural Strength
  • Hardness*
  • Materials Testing*
  • Methacrylates* / chemistry
  • Spectrum Analysis, Raman

Substances

  • Composite Resins
  • Methacrylates
  • Bisphenol A-Glycidyl Methacrylate