Activity concentration of indoor radon and its short-lived progeny (218Po, 214Pb, and 214Po) and their effect on atmospheric ionization rate in Sana'a, Yemen

Environ Pollut. 2024 Oct 1:358:124518. doi: 10.1016/j.envpol.2024.124518. Epub 2024 Jul 9.

Abstract

Exposure to ionizing radiation inside houses, especially radionuclides of radon and its progeny, poses serious health risks that can be exacerbated when inhaled as a result of interaction with human lung tissue. Also, air ionization is mainly due to these radionuclides. Therefore, accurate measurements of radon activity concentrations and its short-lived progeny are required to assess dose and environmental pollution and estimate ionization rates in indoor environments. For this purpose, we employed a previously tested and approved reliable method, following the three-count procedure. This method is based on airborne radon progeny sampling on polycarbonate membrane filters and alpha counting using a passive α-dosimetry technique with CR-39 detectors. The method also relies on a PC-based software we developed for solving mathematical equations and calculating all the necessary physical quantities. In this study, the concentrations of radon and individual short-lived radon progeny were measured in 20 houses in Sana'a, Yemen. Measurement conditions and meteorological variables were considered. The average activity concentrations of 222Rn, Equilibrium-Equivalent Concentration (EEC), 218Po, 214 Pb, and 214Po were 73.1 ± 6.0, 29.2 ± 2.4, 44.4 ± 3.6, 30.5 ± 2.5, and 23.2 ± 1.9 Bq.m-3, respectively. The calculated average unattached fractions f1(218Po), f2(214 Pb), and fp were found to be 0.24, 0.04, and 0.07 % respectively. The annual average values of ion-pair production rate caused by 222Rn and their progeny and air ion concentration, were 27.25 ions.cm-3s-1 and 1829 ions.cm-3 respectively. The annual effective dose was estimated to be 1.93 ± 0.16 mSv.y-1, well lower than the recommended 10 mSv.y-1.

Keywords: Air ion concentration; Air ionization; Environmental pollution; Individual short-lived radon progeny; Ion-pair production rate; Radon activity concentration; Unattached fractions.

MeSH terms

  • Air Pollutants, Radioactive* / analysis
  • Air Pollution, Indoor* / analysis
  • Air Pollution, Indoor* / statistics & numerical data
  • Housing
  • Lead Radioisotopes / analysis
  • Polonium / analysis
  • Radiation Monitoring* / methods
  • Radon Daughters* / analysis
  • Radon* / analysis
  • Yemen

Substances

  • Radon
  • Air Pollutants, Radioactive
  • Radon Daughters
  • Polonium
  • Lead Radioisotopes
  • Polonium-210