Evaluation of pharmacokinetics, safety, and efficacy of [211At] meta-astatobenzylguanidine ([211At] MABG) in patients with pheochromocytoma or paraganglioma (PPGL): A study protocol

PLoS One. 2024 May 28;19(5):e0303623. doi: 10.1371/journal.pone.0303623. eCollection 2024.

Abstract

Background: Pheochromocytoma, or paraganglioma (PPGL), is a tumor that arises from catecholamine-producing chromaffin cells of the adrenal medulla or paraganglion. Systemic therapy, such as the combination of cyclophosphamide, vincristine, and dacarbazine or therapeutic radiopharmaceuticals such as [131I] meta-iodobenzylguanidine (MIBG), may be administered in cases of locally advanced tumors or distant metastases. However, the current therapies are limited in terms of efficacy and implementation. [211At] meta-astatobenzylguanidine (MABG) is an alpha-emitting radionuclide-labeled ligand that has demonstrated remarkable tumor-reducing effects in preclinical studies, and is expected to have a high therapeutic effect on pheochromocytoma cells.

Methods: We are currently conducting an investigator-initiated first-in-human clinical trial to evaluate the pharmacokinetics, safety, and efficacy of [211At] MABG. Patients with locally unresectable or metastatic PPGL refractory to standard therapy and scintigraphically positive [123I] MIBG aggregation are being recruited, and a 3 + 3 dose escalation design was adopted. The initial dose of [211At] MABG is 0.65 MBq/kg, with a dose escalation in a 1:2:4 ratio in each cohort. Dose-limiting toxicity is observed for 6 weeks after a single bolus dose of [211At] MABG, and the patients are observed for 3 months to explore safety and efficacy profiles. The primary endpoint is dose-limiting toxicity to determine both maximum tolerated and recommended doses. The secondary endpoints include radiopharmacokinetics, urinary radioactive excretion rate, urinary catecholamine response rate, objective response rate, progression free survival, [123I] MIBG scintigraphy on reducing tumor accumulation, and quality of life.

Trials registration: jRCT2021220012 registered on 17 June 2022.

Publication types

  • Clinical Trial Protocol

MeSH terms

  • Adrenal Gland Neoplasms* / diagnostic imaging
  • Adrenal Gland Neoplasms* / drug therapy
  • Adrenal Gland Neoplasms* / metabolism
  • Adrenal Gland Neoplasms* / pathology
  • Adult
  • Aged
  • Clinical Trials, Phase I as Topic
  • Female
  • Guanidines / pharmacokinetics
  • Guanidines / therapeutic use
  • Humans
  • Male
  • Middle Aged
  • Paraganglioma* / diagnostic imaging
  • Paraganglioma* / drug therapy
  • Paraganglioma* / metabolism
  • Paraganglioma* / pathology
  • Pheochromocytoma* / diagnostic imaging
  • Pheochromocytoma* / drug therapy
  • Pheochromocytoma* / metabolism
  • Pheochromocytoma* / pathology
  • Radiopharmaceuticals* / pharmacokinetics
  • Treatment Outcome

Substances

  • Guanidines
  • Radiopharmaceuticals

Grants and funding

This study is funded by the Advanced Clinical Research Center management business subsidy from Japanese government and granted by the Japan Agency for Medical Research and Development(23ck0106815h0001). The funders did not and will not have a role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.