Synergetic effect of lytic polysaccharide monooxygenase from Thermobifida fusca on saccharification of agrowastes

Bioresour Technol. 2023 Jun:378:129015. doi: 10.1016/j.biortech.2023.129015. Epub 2023 Apr 3.

Abstract

Saccharification is one of the most noteworthy processes in biomass-based biorefineries. In particular, the lytic polysaccharide monooxygenase has recently emerged as an oxidative cleavage-recalcitrant polysaccharide; however, there is insufficient information regarding its application to actual biomass. Accordingly, this study focused optimizing the recombinant expression level of a bacterial lytic polysaccharide monooxygenase from Thermobifida fusca (TfLPMO), which was characterized as a cellulolytic enzyme. Finally, the synergistic effect of the lytic polysaccharide monooxygenase and a commercial cellulase cocktail on the saccharification of agrowaste was investigated. TfLPMO functioned on various cellulosic and hemicellulosic substrates, and the combination of TfLPMO with cellulase exhibited a synergistic effect on the saccharification of agrowastes, resulting in a 19.2% and 14.1% increase in reducing sugars from rice straw and corncob, respectively. The results discussed herein can lead to an in-depth understanding of enzymatic saccharification and suggest viable options for valorizing agrowastes as renewable feedstocks in biorefineries.

Keywords: Agricultural waste; LPMO from Thermobifida fusca; Recombinant expression; Synergistic effect with cellulase.

MeSH terms

  • Cellulase* / metabolism
  • Mixed Function Oxygenases* / metabolism
  • Polysaccharides / metabolism

Substances

  • Mixed Function Oxygenases
  • Polysaccharides
  • Cellulase

Supplementary concepts

  • Thermobifida fusca