Tumor oxygenation nanoliposome synergistic hypoxia-inducible-factor-1 inhibitor enhanced Iodine-125 seed brachytherapy for esophageal cancer

Biomaterials. 2022 Oct:289:121801. doi: 10.1016/j.biomaterials.2022.121801. Epub 2022 Sep 13.

Abstract

Iodine-125 (125I) brachytherapy has become one of the most effective palliative treatment options for advanced esophageal cancer. However, resistance toward 125I brachytherapy caused by pre-existing tumor hypoxia and hypoxia-inducible factor 1 (HIF-1) signaling pathway activation represents a significant limitation in esophageal cancer treatment. To circumvent these problems, herein, we proposed an innovative strategy to alleviate radioresistance of brachytherapy by co-encapsulating catalase (CAT) and HIF-1 inhibitor-acriflavine (ACF) into the hydrophilic cavities of liposome, termed as "ACF-CAT@Lipo". Under overexpressed H2O2 stimulation in the tumor region, the fabricated ACF-CAT@Lipo can generate an amount of O2 and alleviate tumor hypoxia in vitro and in vivo. Furthermore, cooperating with ACF, the expression of hypoxia-related protein (e.g. HIF-1α, VEGF, MMP-2) are obviously decreased. Importantly, the copious oxygenation and the significant inhibition expression of HIF-1α can further improve the radiosensitivity of 125I brachytherapy and finally realize the eradication of esophageal cancer in vivo. The oxygen enrichment and HIF-1 inhibition function of ACF-CAT@Lipo provides a new strategy to overcome the brachytherapy resistance of esophageal cancer therapy.

Keywords: (125)I brachytherapy; Esophageal cancer; HIF-1 functional inhibition; Radiosensitizer; Tumor hypoxia.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acriflavine / pharmacology
  • Brachytherapy*
  • Catalase
  • Cell Line, Tumor
  • Esophageal Neoplasms* / drug therapy
  • Esophageal Neoplasms* / metabolism
  • Esophageal Neoplasms* / radiotherapy
  • Humans
  • Hydrogen Peroxide
  • Hypoxia
  • Hypoxia-Inducible Factor 1
  • Hypoxia-Inducible Factor 1, alpha Subunit
  • Iodine Radioisotopes
  • Liposomes
  • Matrix Metalloproteinase 2
  • Oxygen / metabolism
  • Vascular Endothelial Growth Factor A

Substances

  • Hypoxia-Inducible Factor 1
  • Hypoxia-Inducible Factor 1, alpha Subunit
  • Iodine Radioisotopes
  • Liposomes
  • Vascular Endothelial Growth Factor A
  • Acriflavine
  • Hydrogen Peroxide
  • Catalase
  • Matrix Metalloproteinase 2
  • Iodine-125
  • Oxygen