PhI(OAc)2-mediated trifluoromethylthiolation/oxidative cyclization of ynamides

Org Biomol Chem. 2021 Oct 20;19(40):8746-8753. doi: 10.1039/d1ob01642c.

Abstract

A PhI(OAc)2-mediated trifluoromethylthiolation/oxidative cyclization of ynamides with the Shen reagent has been established herein, providing a facile access to CF3S-substituted oxazolidine-2,4-diones bearing a quaternary carbon center in 38-85% yields with chemoselectivities of up to 99/1.

Publication types

  • Research Support, Non-U.S. Gov't