Mitochondrial metabolism supports resistance to IDH mutant inhibitors in acute myeloid leukemia

J Exp Med. 2021 May 3;218(5):e20200924. doi: 10.1084/jem.20200924.

Abstract

Mutations in IDH induce epigenetic and transcriptional reprogramming, differentiation bias, and susceptibility to mitochondrial inhibitors in cancer cells. Here, we first show that cell lines, PDXs, and patients with acute myeloid leukemia (AML) harboring an IDH mutation displayed an enhanced mitochondrial oxidative metabolism. Along with an increase in TCA cycle intermediates, this AML-specific metabolic behavior mechanistically occurred through the increase in electron transport chain complex I activity, mitochondrial respiration, and methylation-driven CEBPα-induced fatty acid β-oxidation of IDH1 mutant cells. While IDH1 mutant inhibitor reduced 2-HG oncometabolite and CEBPα methylation, it failed to reverse FAO and OxPHOS. These mitochondrial activities were maintained through the inhibition of Akt and enhanced activation of peroxisome proliferator-activated receptor-γ coactivator-1 PGC1α upon IDH1 mutant inhibitor. Accordingly, OxPHOS inhibitors improved anti-AML efficacy of IDH mutant inhibitors in vivo. This work provides a scientific rationale for combinatory mitochondrial-targeted therapies to treat IDH mutant AML patients, especially those unresponsive to or relapsing from IDH mutant inhibitors.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acute Disease
  • Aminopyridines / pharmacology
  • Animals
  • Cell Line, Tumor
  • Doxycycline / pharmacology
  • Drug Resistance, Neoplasm / drug effects
  • Drug Resistance, Neoplasm / genetics*
  • Enzyme Inhibitors / pharmacology
  • Epigenesis, Genetic / drug effects
  • Glycine / analogs & derivatives
  • Glycine / pharmacology
  • HL-60 Cells
  • Humans
  • Isocitrate Dehydrogenase / antagonists & inhibitors
  • Isocitrate Dehydrogenase / genetics*
  • Isocitrate Dehydrogenase / metabolism
  • Isoenzymes / antagonists & inhibitors
  • Isoenzymes / genetics
  • Isoenzymes / metabolism
  • Leukemia, Myeloid / drug therapy
  • Leukemia, Myeloid / genetics*
  • Leukemia, Myeloid / metabolism
  • Mice
  • Mice, Inbred NOD
  • Mice, Knockout
  • Mice, SCID
  • Mitochondria / drug effects
  • Mitochondria / genetics*
  • Mitochondria / metabolism
  • Mutation*
  • Oxadiazoles / pharmacology
  • Oxidative Phosphorylation / drug effects
  • Piperidines / pharmacology
  • Pyridines / pharmacology
  • Triazines / pharmacology
  • Xenograft Model Antitumor Assays / methods

Substances

  • Aminopyridines
  • Enzyme Inhibitors
  • IACS-010759
  • Isoenzymes
  • Oxadiazoles
  • Piperidines
  • Pyridines
  • Triazines
  • enasidenib
  • Isocitrate Dehydrogenase
  • Doxycycline
  • ivosidenib
  • Glycine