Decoding the protein composition of whole nucleosomes with Nuc-MS

Nat Methods. 2021 Mar;18(3):303-308. doi: 10.1038/s41592-020-01052-9. Epub 2021 Feb 15.

Abstract

Current proteomic approaches disassemble and digest nucleosome particles, blurring readouts of the 'histone code'. To preserve nucleosome-level information, we developed Nuc-MS, which displays the landscape of histone variants and their post-translational modifications (PTMs) in a single mass spectrum. Combined with immunoprecipitation, Nuc-MS quantified nucleosome co-occupancy of histone H3.3 with variant H2A.Z (sixfold over bulk) and the co-occurrence of oncogenic H3.3K27M with euchromatic marks (for example, a >15-fold enrichment of dimethylated H3K79me2). Nuc-MS is highly concordant with chromatin immunoprecipitation-sequencing (ChIP-seq) and offers a new readout of nucleosome-level biology.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cell Line
  • Chromatin Immunoprecipitation / methods
  • HEK293 Cells
  • Histone Code
  • Histones / metabolism*
  • Humans
  • Methylation
  • Nucleosomes / metabolism*
  • Proteomics / methods*
  • Spectrometry, Mass, Electrospray Ionization / methods*

Substances

  • Histones
  • Nucleosomes