The Effect of 4-Methylpyrazole on Oxidative Metabolism of Acetaminophen in Human Volunteers

J Med Toxicol. 2020 Apr;16(2):169-176. doi: 10.1007/s13181-019-00740-z. Epub 2019 Nov 25.

Abstract

Introduction: Acetaminophen (APAP) is commonly ingested in both accidental and suicidal overdose. Oxidative metabolism by cytochrome P450 2E1 (CYP2E1) produces the hepatotoxic metabolite, N-acetyl-p-benzoquinone imine. CYP2E1 inhibition using 4-methylpyrazole (4-MP) has been shown to prevent APAP-induced liver injury in mice and human hepatocytes. This study was conducted to assess the effect of 4-MP on APAP metabolism in humans.

Methods: This crossover trial examined the ability of 4-MP to inhibit CYP2E1 metabolism of APAP in five human volunteers. Participants received a single oral dose of APAP 80 mg/kg, both with and without intravenous 4-MP, after which urinary and plasma oxidative APAP metabolites were measured. The primary outcome was the fraction of ingested APAP excreted as total oxidative metabolites (APAP-CYS, APAP-NAC, APAP-GSH).

Results: Compared with APAP alone, co-treatment with 4-MP decreased the percentage of ingested APAP recovered as oxidative metabolites in 24-hour urine from 4.48 to 0.51% (95% CI = 2.31-5.63%, p = 0.003). Plasma concentrations of these oxidative metabolites also decreased.

Conclusions: These results show 4-MP effectively reduced oxidative metabolism of APAP in human volunteers ingesting a supratherapeutic APAP dose.

Trial registration: ClinicalTrials.gov Identifier: NCT03878693.

Keywords: 4-Methylpyrazole; Acetaminophen toxicity; CYP2E1; Hepatotoxicity; Overdose.

Publication types

  • Randomized Controlled Trial
  • Research Support, N.I.H., Extramural

MeSH terms

  • Acetaminophen / administration & dosage
  • Acetaminophen / pharmacokinetics*
  • Activation, Metabolic
  • Administration, Oral
  • Adult
  • Analgesics, Non-Narcotic / administration & dosage
  • Analgesics, Non-Narcotic / pharmacokinetics*
  • Cross-Over Studies
  • Cytochrome P-450 CYP2E1 / metabolism*
  • Cytochrome P-450 CYP2E1 Inhibitors / administration & dosage*
  • Drug Interactions
  • Female
  • Fomepizole / administration & dosage*
  • Humans
  • Infusions, Intravenous
  • Male
  • Middle Aged
  • Oxidation-Reduction

Substances

  • Analgesics, Non-Narcotic
  • Cytochrome P-450 CYP2E1 Inhibitors
  • Acetaminophen
  • Fomepizole
  • Cytochrome P-450 CYP2E1

Associated data

  • ClinicalTrials.gov/NCT03878693