Hyaluronic Acid-Decorated Liposomes as Innovative Targeted Delivery System for Lung Fibrotic Cells

Molecules. 2019 Sep 10;24(18):3291. doi: 10.3390/molecules24183291.

Abstract

Collagen Tissue Disease-associated Interstitial Lung Fibrosis (CTD-ILDs) and Bronchiolitis Obliterans Syndrome (BOS) represent severe lung fibrogenic disorders, characterized by fibro-proliferation with uncontrolled extracellular matrix deposition. Hyaluronic acid (HA) plays a key role in fibrosis with its specific receptor, CD44, overexpressed by CTD-ILD and BOS cells. The aim is to use HA-liposomes to develop an inhalatory treatment for these diseases. Liposomes with HA of two molecular weights were prepared and characterized. Targeting efficiency was assessed toward CTD-ILD and BOS cells by flow cytometry and confocal microscopy and immune modulation by RT-PCR and ELISA techniques. HA-liposomes were internalized by CTD-ILD and BOS cells expressing CD44, and this effect increased with higher HA MW. In THP-1 cells, HA-liposomes decreased pro-inflammatory cytokines IL-1β, IL-12, and anti-fibrotic VEGF transcripts but increased TGF-β mRNA. However, upon analyzing TGF-β release from healthy donors-derived monocytes, we found liposomes did not alter the release of active pro-fibrotic cytokine. All liposomes induced mild activation of neutrophils regardless of the presence of HA. HA liposomes could be also applied for lung fibrotic diseases, being endowed with low pro-inflammatory activity, and results confirmed that higher MW HA are associated to an increased targeting efficiency for CD44 expressing LFs-derived from BOS and CTD-ILD patients.

Keywords: Bronchiolitis Obliterans Syndrome; hyaluronic acid; immune cells; liposomes; lung fibrosis.

MeSH terms

  • A549 Cells
  • Adult
  • Bronchiolitis Obliterans / drug therapy*
  • Bronchiolitis Obliterans / pathology
  • Drug Delivery Systems
  • Gene Expression Regulation / drug effects
  • Healthy Volunteers
  • Humans
  • Hyaluronan Receptors / drug effects
  • Hyaluronic Acid / chemistry
  • Hyaluronic Acid / pharmacology*
  • Liposomes / chemistry
  • Liposomes / pharmacology*
  • Microscopy, Confocal
  • Monocytes / drug effects
  • Pulmonary Fibrosis / drug therapy*
  • Pulmonary Fibrosis / pathology
  • Transforming Growth Factor beta / genetics
  • Vascular Endothelial Growth Factor A / genetics

Substances

  • CD44 protein, human
  • Hyaluronan Receptors
  • Liposomes
  • Transforming Growth Factor beta
  • VEGFA protein, human
  • Vascular Endothelial Growth Factor A
  • Hyaluronic Acid