A 3D printed chitosan-pectin hydrogel wound dressing for lidocaine hydrochloride delivery

Mater Sci Eng C Mater Biol Appl. 2019 Nov:104:109873. doi: 10.1016/j.msec.2019.109873. Epub 2019 Jun 8.

Abstract

A chitosan-pectin (CS-PEC) biopolymeric hydrogel wound dressing was investigated for lidocaine delivery. Here we demonstrate for the first time the feasibility of three-dimensional (3D) printed CS-PEC hydrogel incorporating the local anaesthetic drug lidocaine hydrochloride (LDC) as a potential wound dressing candidate. The hydrogels were prepared by physical crosslinking of CS and PEC polysaccharides. The scaffolds were printed using an extrusion-based 3D printer using a mechanical positive displacement dispensing system followed by lyophilisation. The 3D printed hydrogels showed good printability, dimensional integrity and self-adhesion to skin. The high swelling ratio and water absorption of 3D printed hydrogels indicated suitability for absorbing exudates and maintaining a moist wound healing environment. Fourier transform infrared (FTIR) spectroscopy results indicated that the CS-PEC hydrogel was formed by hydrogen bonds. Incorporation of LDC in the hydrogel did not interfere with its functional stability. In vitro drug release studies of LDC over 6 h fitted the Korsmeyer-Peppas model. This work demonstrates the possibility of a 3D printed hydrogel as a suitable candidate for wound dressings.

Keywords: 3D printing; Chitosan; Hydrogel; Lidocaine hydrochloride; Pectin; Wound dressing.

MeSH terms

  • Adhesiveness
  • Bandages*
  • Calorimetry, Differential Scanning
  • Chitosan / chemistry*
  • Drug Delivery Systems*
  • Drug Liberation
  • Feasibility Studies
  • Hydrogels / chemistry*
  • Kinetics
  • Lidocaine / pharmacology*
  • Pectins / chemistry*
  • Printing, Three-Dimensional*
  • Spectroscopy, Fourier Transform Infrared
  • Tissue Scaffolds / chemistry
  • Water

Substances

  • Hydrogels
  • Water
  • Pectins
  • Chitosan
  • Lidocaine