Chemical Control over T-Cell Activation in Vivo Using Deprotection of trans-Cyclooctene-Modified Epitopes

ACS Chem Biol. 2018 Jun 15;13(6):1569-1576. doi: 10.1021/acschembio.8b00155. Epub 2018 May 11.

Abstract

Activation of a cytotoxic T-cell is a complex multistep process, and tools to study the molecular events and their dynamics that result in T-cell activation in situ and in vivo are scarce. Here, we report the design and use of conditional epitopes for time-controlled T-cell activation in vivo. We show that trans-cyclooctene-protected SIINFEKL (with the lysine amine masked) is unable to elicit the T-cell response characteristic for the free SIINFEKL epitope. Epitope uncaging by means of an inverse-electron demand Diels-Alder (IEDDA) event restored T-cell activation and provided temporal control of T-cell proliferation in vivo.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cell Line
  • Cycloaddition Reaction
  • Cyclooctanes / chemical synthesis
  • Cyclooctanes / immunology*
  • Dendritic Cells / immunology
  • Epitopes / chemistry
  • Epitopes / immunology*
  • Female
  • Heterocyclic Compounds, 1-Ring / chemistry
  • Lymphocyte Activation / drug effects*
  • Mice, Inbred C57BL
  • T-Lymphocytes, Cytotoxic / immunology*

Substances

  • Cyclooctanes
  • Epitopes
  • Heterocyclic Compounds, 1-Ring