Characterization of minoxidil/hydroxypropyl-β-cyclodextrin inclusion complex in aqueous alginate gel useful for alopecia management: Efficacy evaluation in male rat

Eur J Pharm Biopharm. 2018 Jan:122:146-157. doi: 10.1016/j.ejpb.2017.10.015. Epub 2017 Oct 24.

Abstract

Solid inclusion complex between hydroxypropyl-β-cyclodextrin (HP-β-CD) and minoxidil (MXD) was prepared by freeze-drying and characterized by yield, drug loading and dissolution rate. Moreover, the complex was formulated as alginate gel (GEL HP-β-CD)/MXD 3.5% w/w). The efficacy of the novel GEL HP-β-CD)/MXD 3.5% w/w and of MXD 3.5% w/w ethanolic/propylene-glycol solution (MXD solution) were evaluated by monitoring the hair growth of dorsal skin 1-4 weeks after depilation followed by histological analysis and gene expression in skin biopsies in male rat. Patch-clamp experiments and cell-dehydrogenase activity (CDA) were performed to evaluate the capability of the formulations to activate "in vitro" the ATP-sensitive K+-channels (KATP) and their effects on cell viability in skin fibroblasts. After 3 weeks, the MXD solution and MXD/HP-β-CD GEL enhanced the hair growth, respectively, of 80.1 ± 2% and 84.3 ± 4% vs controls. After 4 weeks, the MXD/HP-β-CD GEL significantly enhanced the hair length and bulb diameter vs others groups. The MXD/HP-β-CD GEL significantly enhanced the mRNA levels of the SUR2 and Kir6.1 subunits of the KATP channels and AKT2 vs other groups. The AR gene was down-regulated vs controls following the treatment with either MXD formulations. Either MXD (10-4 M) formulations were effective in potentiating the KATP currents. The MXD solution and its vehicle after 9 h of incubation time, but not MXD/HP-β-CD, reduced CDA in fibroblasts. In sum, the MXD/HP-β-CD GEL shows a favorable profile following topical long-term use.

Keywords: Alopecia; Barium ions (PubChem CID: 24414); Ethanol (PubChem CID: 702); GEL formulation; Gene expression; Glybenclamide (PubChem CID: 3488); Hair growth; Hydroxylpropyl-β-cyclodextrin; Hydroxypropil beta cyclodextrin (PubChem CID: 44134771); Inclusion complex; KATP channels; Minoxidil; Minoxidil (PubChem CID: 4201); Propylene glycol (PubChem CID: 174); Tetraethylammonium (TEA) (PubChem CID: 5413).

MeSH terms

  • 2-Hydroxypropyl-beta-cyclodextrin / chemistry
  • 2-Hydroxypropyl-beta-cyclodextrin / pharmacology*
  • Administration, Topical
  • Alginates / chemistry
  • Alginates / pharmacology*
  • Alopecia / drug therapy*
  • Alopecia / metabolism
  • Animals
  • Chemistry, Pharmaceutical / methods
  • Drug Carriers / chemistry
  • Excipients / chemistry
  • Fibroblasts / drug effects
  • Gels / chemistry
  • Gels / pharmacology*
  • Glucuronic Acid / chemistry
  • Glucuronic Acid / pharmacology
  • Hair / drug effects
  • Hair / metabolism
  • Hexuronic Acids / chemistry
  • Hexuronic Acids / pharmacology
  • KATP Channels / metabolism
  • Male
  • Minoxidil / chemistry
  • Minoxidil / pharmacology*
  • Rats
  • Rats, Wistar
  • Skin / metabolism
  • Skin Absorption / drug effects
  • Solubility / drug effects
  • Water / chemistry

Substances

  • Alginates
  • Drug Carriers
  • Excipients
  • Gels
  • Hexuronic Acids
  • KATP Channels
  • Water
  • 2-Hydroxypropyl-beta-cyclodextrin
  • Minoxidil
  • Glucuronic Acid