Probucol ameliorates renal injury in diabetic nephropathy by inhibiting the expression of the redox enzyme p66Shc

Redox Biol. 2017 Oct:13:482-497. doi: 10.1016/j.redox.2017.07.002. Epub 2017 Jul 4.

Abstract

Aims: Probucol is an anti-hyperlipidemic agent and a potent antioxidant drug that can delay progression of diabetic nephropathy (DN) and reverses renal oxidative stress in diabetic animal models; however, the mechanisms underlying these effects remain unclear. p66Shc is a newly recognized mediator of mitochondrial ROS production in renal cells under high-glucose (HG) ambience. We previously showed that p66Shc can serve as a biomarker for renal oxidative injury in DN patients and that p66Shc up-regulation is correlated with renal damage in vivo and in vitro. Here, we determined whether probucol ameliorates renal injury in DN by inhibiting p66Shc expression.

Results: We found that the expression of SIRT1, Ac-H3 and p66Shc in kidneys of DN patients was altered. Also, probucol reduced the levels of serum creatinine, urine protein and LDL-c and attenuated renal oxidative injury and fibrosis in STZ induced diabetic mice. In addition, probucol reversed p-AMPK, SIRT1, Ac-H3 and p66Shc expression. Correlation analyses showed that p66Shc expression was correlated with p-AMPK and Sirt1 expression and severity of renal injury. In vitro pretreatment of HK-2 cells with p-AMPK and SIRT1 siRNA negated the beneficial effects of probucol. Furthermore, we noted that probucol activates p-AMPK and Sirt1 and inhibits p66shc mRNA transcription by facilitating the binding of Sirt1 to the p66Shc promoter and modulation of Ac-H3 expression in HK-2 cells under HG ambience.

Innovation and conclusion: Our results suggest for the first time that probucol ameliorates renal damage in DN by epigenetically suppressing p66Shc expression via the AMPK-SIRT1-AcH3 pathway.

Keywords: Diabetic nephropathy; Probucol; Renal injury; p66Shc.

MeSH terms

  • AMP-Activated Protein Kinase Kinases
  • Animals
  • Anticholesteremic Agents / pharmacology*
  • Anticholesteremic Agents / therapeutic use
  • Antioxidants / pharmacology*
  • Antioxidants / therapeutic use
  • Cell Line
  • Diabetic Nephropathies / drug therapy*
  • Diabetic Nephropathies / metabolism
  • Histones / metabolism
  • Humans
  • Kidney / drug effects
  • Kidney / metabolism
  • Mice
  • Mice, Inbred C57BL
  • Probucol / pharmacology*
  • Probucol / therapeutic use
  • Protein Kinases / genetics
  • Protein Kinases / metabolism
  • Sirtuin 1 / genetics
  • Sirtuin 1 / metabolism
  • Src Homology 2 Domain-Containing, Transforming Protein 1 / antagonists & inhibitors*
  • Src Homology 2 Domain-Containing, Transforming Protein 1 / genetics
  • Src Homology 2 Domain-Containing, Transforming Protein 1 / metabolism

Substances

  • Anticholesteremic Agents
  • Antioxidants
  • Histones
  • Shc1 protein, mouse
  • Src Homology 2 Domain-Containing, Transforming Protein 1
  • Protein Kinases
  • AMP-Activated Protein Kinase Kinases
  • Sirt1 protein, mouse
  • Sirtuin 1
  • Probucol