Remote Photoregulated Ring Gliding in a [2]Rotaxane via a Molecular Effector

Org Lett. 2017 Jan 6;19(1):154-157. doi: 10.1021/acs.orglett.6b03457. Epub 2016 Dec 9.

Abstract

A molecular barbiturate messenger, which is reversibly released/captured by a photoswitchable artificial molecular receptor, is shown to act as an effector to control ring gliding on a distant hydrogen-bonding [2]rotaxane. Thus, light-driven chemical communication governing the operation of a remote molecular machine is demonstrated using an information-rich neutral molecule.

Publication types

  • Research Support, Non-U.S. Gov't