Anti-vascular inflammatory effects of pentacyclic triterpenoids from Astilbe rivularis in vitro and in vivo

Chem Biol Interact. 2017 Jan 5:261:127-138. doi: 10.1016/j.cbi.2016.11.014. Epub 2016 Nov 22.

Abstract

Sepsis is a systemic inflammatory condition resulting from bacterial infections. It is associated with high mortality rates, and its therapeutic options are limited. Transforming growth factor β induced protein (TGFBIp) is an extracellular matrix protein that functions as a mediator of experimental sepsis. C-27-carboxylated pentacyclic triterpenoids are specifically found in species of the genus Astilbe, and show several biological effects. Given the anti-inflammatory effects of pentacyclic triterpenoids, we investigated the effects of 3β-trans-p-coumaroyloxy-olean-12-en-27-oic acid (1) and 6β-hydroxy-3-oxoolean-12-en-27-oic acid (2) on TGFBIp-mediated vascular inflammatory responses. The anti-inflammatory activities of compounds 1 and 2 were determined by measuring the permeability, leukocyte adhesion and migration, and activation of pro-inflammatory proteins in TGFBIp-activated human umbilical vein endothelial cells (HUVECs) and mice. We found that compounds 1 and 2 inhibited lipopolysaccharide (LPS)-induced TGFBIp secretion, TGFBIp-induced barrier disruption, expression of cell adhesion molecules (CAMs), and the adhesion/transendothelial migration of the neutrophils to the human endothelial cells. Compounds 1 and 2 also suppressed TGFBIp-induced hyperpermeability and leukocyte migration in vivo. These results suggested that C-27-carboxylated pentacyclic triterpenoids 1 and 2 have anti-inflammatory functions by inhibiting hyperpermeability, CAM expression, and leukocyte adhesion/migration. Therefore, these compounds can be considered as a potential therapy for vascular inflammatory diseases.

Keywords: Astilbe rivularis; C-27 Carboxylated pentacyclic triterpenoids; Inflammation; Sepsis; TGFBIp.

MeSH terms

  • Animals
  • Anti-Inflammatory Agents / chemistry
  • Anti-Inflammatory Agents / pharmacology*
  • Anti-Inflammatory Agents / therapeutic use
  • Cecum / pathology
  • Cell Adhesion / drug effects
  • Cell Adhesion Molecules / metabolism
  • Cell Movement / drug effects
  • Extracellular Matrix Proteins / metabolism
  • Human Umbilical Vein Endothelial Cells / drug effects
  • Human Umbilical Vein Endothelial Cells / pathology
  • Humans
  • Inflammation / pathology
  • Interleukin-6 / metabolism
  • Ligation
  • Lipopolysaccharides / pharmacology
  • Lung / drug effects
  • Lung / pathology
  • Male
  • Mice, Inbred C57BL
  • NF-kappa B / metabolism
  • Neutrophils / cytology
  • Neutrophils / drug effects
  • Pentacyclic Triterpenes / chemistry
  • Pentacyclic Triterpenes / pharmacology*
  • Pentacyclic Triterpenes / therapeutic use
  • Permeability / drug effects
  • Protective Agents / pharmacology
  • Protective Agents / therapeutic use
  • Punctures
  • Saxifragaceae / chemistry*
  • Sepsis / drug therapy
  • Sepsis / pathology
  • Transforming Growth Factor beta / metabolism
  • Tumor Necrosis Factor-alpha / metabolism

Substances

  • Anti-Inflammatory Agents
  • Cell Adhesion Molecules
  • Extracellular Matrix Proteins
  • Interleukin-6
  • Lipopolysaccharides
  • NF-kappa B
  • Pentacyclic Triterpenes
  • Protective Agents
  • Transforming Growth Factor beta
  • Tumor Necrosis Factor-alpha
  • betaIG-H3 protein