Integrated Computational Solution for Predicting Skin Sensitization Potential of Molecules

PLoS One. 2016 Jun 7;11(6):e0155419. doi: 10.1371/journal.pone.0155419. eCollection 2016.

Abstract

Introduction: Skin sensitization forms a major toxicological endpoint for dermatology and cosmetic products. Recent ban on animal testing for cosmetics demands for alternative methods. We developed an integrated computational solution (SkinSense) that offers a robust solution and addresses the limitations of existing computational tools i.e. high false positive rate and/or limited coverage.

Results: The key components of our solution include: QSAR models selected from a combinatorial set, similarity information and literature-derived sub-structure patterns of known skin protein reactive groups. Its prediction performance on a challenge set of molecules showed accuracy = 75.32%, CCR = 74.36%, sensitivity = 70.00% and specificity = 78.72%, which is better than several existing tools including VEGA (accuracy = 45.00% and CCR = 54.17% with 'High' reliability scoring), DEREK (accuracy = 72.73% and CCR = 71.44%) and TOPKAT (accuracy = 60.00% and CCR = 61.67%). Although, TIMES-SS showed higher predictive power (accuracy = 90.00% and CCR = 92.86%), the coverage was very low (only 10 out of 77 molecules were predicted reliably).

Conclusions: Owing to improved prediction performance and coverage, our solution can serve as a useful expert system towards Integrated Approaches to Testing and Assessment for skin sensitization. It would be invaluable to cosmetic/ dermatology industry for pre-screening their molecules, and reducing time, cost and animal testing.

MeSH terms

  • Animals
  • Computer Simulation*
  • Drug Evaluation, Preclinical / methods
  • Humans
  • Models, Biological*
  • Skin* / immunology
  • Skin* / metabolism
  • Skin* / pathology

Grants and funding

All authors are employees of Persistent Systems Limited. The funder provided support in the form of salaries for authors [KK, ST, AD, VS and AJ], but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the ‘author contributions’ section.