Inhibitors of DNA Methylation, Histone Deacetylation, and Histone Demethylation: A Perfect Combination for Cancer Therapy

Adv Cancer Res. 2016:130:55-111. doi: 10.1016/bs.acr.2016.01.007. Epub 2016 Mar 2.

Abstract

Epigenetic silencing and inappropriate activation of gene expression are frequent events during the initiation and progression of cancer. These events involve a complex interplay between the hypermethylation of CpG dinucleotides within gene promoter and enhancer regions, the recruitment of transcriptional corepressors and the deacetylation and/or methylation of histone tails. These epigenetic regulators act in concert to block transcription or interfere with the maintenance of chromatin boundary regions. However, DNA/histone methylation and histone acetylation states are reversible, enzyme-mediated processes and as such, have emerged as promising targets for cancer therapy. This review will focus on the potential benefits and synergistic/additive effects of combining DNA-demethylating agents and histone deacetylase inhibitors or lysine-specific demethylase inhibitors together in epigenetic therapy for solid tumors and will highlight what is known regarding the mechanisms of action that contribute to the antitumor response.

Keywords: DNA methyltransferase inhibitors; Drug synergy; Epigenetic therapy; Histone deacetylation and methylation inhibitors; Solid tumors.

Publication types

  • Review

MeSH terms

  • Antineoplastic Agents / therapeutic use*
  • DNA Methylation / genetics*
  • Drug Synergism
  • Epigenesis, Genetic
  • Histone Deacetylase Inhibitors / therapeutic use*
  • Histone Deacetylases / therapeutic use*
  • Histones / metabolism*
  • Humans
  • Neoplasms / drug therapy*
  • Promoter Regions, Genetic
  • RNA / genetics
  • RNA / metabolism
  • Transcription, Genetic

Substances

  • Antineoplastic Agents
  • Histone Deacetylase Inhibitors
  • Histones
  • RNA
  • Histone Deacetylases