Simultaneous Electro-Optical Tracking for Nanoparticle Recognition and Counting

Nano Lett. 2015 Sep 9;15(9):5696-701. doi: 10.1021/acs.nanolett.5b01243. Epub 2015 Aug 5.

Abstract

We present the first detailed experimental observation and analysis of nanoparticle electrophoresis through a nanochannel obtained with synchronous high-bandwidth electrical and camera recordings. Optically determined particle diffusion coefficients agree with values extracted from fitting electrical transport measurements to distributions from 1D Fokker-Planck diffusion-drift theory. This combined tracking strategy enables optical recognition and electrical characterization of nanoparticles in solution, which can have a broad range of applications in biology and materials science.

Keywords: Single particle tracking; nanoparticle diffusion; polymeric nanochannels; resistive pulse sensing; translocation dynamics.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Diffusion
  • Dimethylpolysiloxanes / chemistry
  • Electrophoresis / instrumentation*
  • Equipment Design
  • Fluorescent Dyes / analysis
  • Lab-On-A-Chip Devices*
  • Nanoparticles / analysis*
  • Nanotechnology / instrumentation
  • Optics and Photonics / instrumentation
  • Particle Size
  • Video Recording

Substances

  • Dimethylpolysiloxanes
  • Fluorescent Dyes
  • baysilon