NMR assignment of intrinsically disordered self-processing module of the FrpC protein of Neisseria meningitidis

Biomol NMR Assign. 2015 Oct;9(2):435-40. doi: 10.1007/s12104-015-9625-z. Epub 2015 Jul 3.

Abstract

The self-processing module (SPM) is an internal segment of the FrpC protein (P415-F591) secreted by the pathogenic Gram-negative bacterium Neisseria meningitidis during meningococcal infection of human upper respiratory tract. SPM mediates 'protein trans-splicing', a unique natural mechanism for editing of proteins, which involves a calcium-dependent autocatalytic cleavage of the peptide bond between D414 and P415 and covalent linkage of the cleaved fragment through its carboxy-terminal group of D414 to [Formula: see text]-amino group of lysine residue within a neighboring polypeptide chain. We present an NMR resonance assignment of the calcium-free SPM, which displays characteristic features of intrinsically disordered proteins. Non-uniformly sampled 5D HN(CA)CONH, 4D HCBCACON, and HCBCANCO spectra were recorded to resolve poorly dispersed resonance frequencies of the disordered protein and 91 % of SPM residues were unambiguously assigned. Analysis of the chemical shifts revealed that two regions of the intrinsically disordered SPM (A95-S101 and R120-I127) have a tendency to form a helical structure, whereas the residues P1-D7 and G36-A40 have the propensity to adopt a [Formula: see text]-structure.

Keywords: FrpC; Intrinsically disordered proteins; Neisseria meningitidis; Resolution-enhanced spectroscopy; Resonance assignment; Self-processing module; Sparse sampling.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bacterial Proteins / chemistry*
  • Intrinsically Disordered Proteins / chemistry*
  • Membrane Proteins / chemistry*
  • Neisseria meningitidis / metabolism*
  • Nuclear Magnetic Resonance, Biomolecular*
  • Protein Structure, Secondary

Substances

  • Bacterial Proteins
  • Intrinsically Disordered Proteins
  • Membrane Proteins
  • frpC protein, Neisseria meningitidis