Reduction-responsive cross-linked stearyl peptide for effective delivery of plasmid DNA

Int J Nanomedicine. 2015 May 8:10:3403-16. doi: 10.2147/IJN.S82413. eCollection 2015.

Abstract

Low efficiency and significant toxicity are the main obstacles to successful gene delivery. We have developed a cationic reduction-responsive vector based on a disulfide cross-linked stearylated polyarginine peptide modified with histidine (C-SHR) for DNA delivery. The structure of the C-SHR was characterized, and the in vitro and in vivo transfection efficiency and cytotoxicity of C-SHR/plasmid DNA complexes were examined. Compared with non-cross-linked stearylated polyarginine peptide (SHR), C-SHR increased the intracellular uptake and dissociation behavior of the complexes. In addition, the gene transfection efficiency of C-SHR/plasmid DNA complexes in HEK293 and HeLa cells was improved and was comparable with that of bPEI-25K/plasmid DNA complexes, and the cytotoxicity of C-SHR was significantly less than that of bPEI-25K. Importantly, the in vivo gene transfection efficiency of C-SHR/plasmid DNA complexes was five fold higher than that of SHR/plasmid DNA complexes, suggesting that C-SHR is an efficient non-viral vector for DNA delivery.

Keywords: DNA delivery; histidine; peptide; polyarginine; reduction-responsive; stearyl.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cations
  • Cross-Linking Reagents / chemistry
  • DNA / administration & dosage*
  • DNA / genetics
  • Disulfides / chemistry
  • Female
  • Gene Transfer Techniques
  • Genetic Vectors / administration & dosage*
  • Genetic Vectors / chemistry
  • HEK293 Cells
  • HeLa Cells
  • Humans
  • Mice, Inbred BALB C
  • Peptides / chemical synthesis
  • Peptides / chemistry*
  • Peptides / toxicity
  • Plasmids / genetics*
  • Transfection / methods*
  • Xenograft Model Antitumor Assays

Substances

  • Cations
  • Cross-Linking Reagents
  • Disulfides
  • Peptides
  • polyarginine
  • DNA