Controlled Release, Intestinal Transport, and Oral Bioavailablity of Paclitaxel Can be Considerably Increased Using Suitably Tailored Pegylated Poly(Anhydride) Nanoparticles

J Pharm Sci. 2015 Sep;104(9):2877-86. doi: 10.1002/jps.24354. Epub 2015 Jan 19.

Abstract

The aim of the work was to evaluate in vitro and in vivo the effect of the addition of poly(ethylene glycol) (PEG) to paclitaxel (PTX)-cyclodextrin poly(anhydride) nanoparticles. For this, PTX in poly(anhydride) nanoparticles complexed with cyclodextrins (either 2-hydroxypropyl-β-cyclodextrin or β-cyclodextrin) and combined with PEG 2000 were prepared by the solvent displacement method. Intestinal permeability in vitro and in vivo pharmacokinetic studies in C57BL/6J mice were performed. Nanoparticle formulations containing PTX increased its apparent permeability through rat intestine in vitro in the Ussing chambers, enhancing its permeability 10-15 times compared with commercial Taxol®. In addition, in pharmacokinetic studies, drug plasma levels were observed for at least 24 h leading to a relative oral bioavailability between 60% and 80% for PTX complexed with cyclodextrin and loaded in pegylated poly(anhydride) nanoparticles after oral gavage. In all, PTX-cyclodextrin complexes encapsulated in pegylated nanoparticles managed to promote the intestinal uptake of the drug displaying sustained plasma levels after oral administration to laboratory animals with a more prolonged plasma profile compared with the formulation with no PEG at all. Therefore, pegylated poly(anhydride) nanoparticles represent a promising carrier for the oral delivery of PTX.

Keywords: bioavailability; controlled release; cyclodextrins; nanoparticles; paclitaxel; pegylation; permeability; transmucosal delivery.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Anhydrides / chemistry*
  • Animals
  • Antineoplastic Agents, Phytogenic / administration & dosage*
  • Antineoplastic Agents, Phytogenic / pharmacokinetics*
  • Area Under Curve
  • Biological Availability
  • Biological Transport
  • Chemistry, Pharmaceutical
  • Cyclodextrins / chemistry
  • Delayed-Action Preparations
  • Drug Carriers
  • Intestinal Absorption
  • Mice
  • Mice, Inbred C57BL
  • Nanoparticles / chemistry*
  • Paclitaxel / administration & dosage*
  • Paclitaxel / pharmacokinetics*
  • Polyethylene Glycols / chemistry*
  • Solubility

Substances

  • Anhydrides
  • Antineoplastic Agents, Phytogenic
  • Cyclodextrins
  • Delayed-Action Preparations
  • Drug Carriers
  • Polyethylene Glycols
  • Paclitaxel