Topically applied phospho-sulindac hydrogel is efficacious and safe in the treatment of experimental arthritis in rats

Pharm Res. 2013 Jun;30(6):1471-82. doi: 10.1007/s11095-012-0953-8. Epub 2013 Mar 13.

Abstract

Purpose: Formulate phospho-sulindac (P-S, OXT-328) in a Pluronic hydrogel to be used as a topical anti-inflammatory agent and study its efficacy, safety and pharmacokinetics in an arthritis model.

Methods: LEW/crlBR rats with Freund's adjuvant-induced arthritis were treated with P-S formulated in Pluronic hydrogel (PSH). We determined the clinical manifestations of arthritis including the locomotor activity of the rats; evaluated joints for inflammation, bone resorption, cartilage damage, COX-2 expression and NF-κB activation; assayed plasma IL-6 and IL-10 levels; and studied the pharmacokinetics of P-S in rats after topical or oral administration.

Results: PSH applied at the onset of arthritis or when arthritis was fully developed, suppressed it by 56-82%, improved the locomotor activity of the rats 2.1-4.4 fold, suppressed synovial inflammation, bone resorption, cartilage damage, NF-κB activation and COX-2 expression but not plasma IL-6 and IL-10 levels. There were no side effects. PSH produced rapidly high local levels of P-S with <14% of P-S reaching the circulation, while orally administered P-S was rapidly metabolized generating much lower joint levels of P-S.

Conclusions: Topical application of PSH is efficacious and safe in the treatment of Freund's adjuvant-induced arthritis; has a favorable pharmacokinetic profile; and likely acts by suppressing key pro-inflammatory signaling pathways.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Administration, Oral
  • Administration, Topical
  • Animals
  • Anti-Inflammatory Agents / administration & dosage
  • Anti-Inflammatory Agents / pharmacokinetics
  • Arthritis, Experimental / blood
  • Arthritis, Experimental / chemically induced
  • Arthritis, Experimental / drug therapy*
  • Arthritis, Experimental / metabolism
  • Bone Resorption / blood
  • Bone Resorption / drug therapy
  • Bone Resorption / metabolism
  • Cartilage / drug effects
  • Cartilage / metabolism
  • Cyclooxygenase 2 / metabolism
  • Disease Models, Animal
  • Female
  • Hydrogel, Polyethylene Glycol Dimethacrylate / administration & dosage*
  • Hydrogel, Polyethylene Glycol Dimethacrylate / pharmacokinetics*
  • Inflammation / blood
  • Inflammation / chemically induced
  • Inflammation / drug therapy
  • Inflammation / metabolism
  • Interleukin-10 / blood
  • Interleukin-10 / metabolism
  • Interleukin-6 / blood
  • Interleukin-6 / metabolism
  • Joints / drug effects
  • Joints / metabolism
  • Motor Activity / drug effects
  • NF-kappa B / metabolism
  • Organophosphorus Compounds / administration & dosage*
  • Organophosphorus Compounds / pharmacokinetics*
  • Rats
  • Rats, Inbred Lew
  • Sulindac / administration & dosage*
  • Sulindac / analogs & derivatives*
  • Sulindac / pharmacokinetics*
  • Synovial Membrane / drug effects
  • Synovial Membrane / metabolism

Substances

  • Anti-Inflammatory Agents
  • Interleukin-6
  • NF-kappa B
  • OXT-328
  • Organophosphorus Compounds
  • Interleukin-10
  • Sulindac
  • Hydrogel, Polyethylene Glycol Dimethacrylate
  • Cyclooxygenase 2
  • Ptgs2 protein, rat