Efficient systemic delivery of siRNA by using high-density lipoprotein-mimicking peptide lipid nanoparticles

Nanomedicine (Lond). 2012 Dec;7(12):1813-25. doi: 10.2217/nnm.12.73. Epub 2012 Jul 26.

Abstract

The main challenge for RNAi therapeutics lies in systemic delivery of siRNA to the correct tissues and transporting them into the cytoplasm of targeted cells, at safe, therapeutic levels. Recently, we developed a high-density lipoprotein-mimicking peptide-phospholipid scaffold (HPPS) and demonstrated its direct cytosolic delivery of siRNA in vitro, thereby bypassing endosomal trapping.

Aim: We investigate the in vivo implementation of HPPS for siRNA delivery.

Method & results: After systemic administration in KB tumor-bearing mice, HPPS prolonged the blood circulation time of cholesterol-modified siRNA (chol-siRNA) by a factor of four, improved its biodistribution and facilitated its uptake in scavenger receptor class B type I overexpressed tumors. For therapeutic targeting to the bcl-2 gene, the HPPS-chol-si-bcl-2 nanoparticles downregulated Bcl-2 protein, induced enhanced apoptosis (2.5-fold) in tumors when compared with controls (saline, HPPS, HPPS-chol-si-scramble and chol-si-bcl-2) and significantly inhibited tumor growth with no adverse effect.

Conclusion: HPPS is a safe, efficient nanocarrier for RNAi therapeutics in vivo.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Biomimetic Materials / adverse effects
  • Biomimetic Materials / chemistry*
  • Genes, bcl-2
  • Genetic Therapy
  • Lipoproteins, HDL / adverse effects
  • Lipoproteins, HDL / chemistry*
  • Mice
  • Mice, Inbred BALB C
  • Mice, Nude
  • Nanoparticles / adverse effects
  • Nanoparticles / chemistry*
  • Neoplasms / genetics
  • Neoplasms / pathology
  • Neoplasms / therapy*
  • Peptides / adverse effects
  • Peptides / chemistry*
  • Phospholipids / adverse effects
  • Phospholipids / chemistry*
  • Proto-Oncogene Proteins c-bcl-2 / genetics
  • RNA Interference
  • RNA, Small Interfering / administration & dosage*
  • RNA, Small Interfering / genetics
  • RNA, Small Interfering / therapeutic use
  • Xenograft Model Antitumor Assays

Substances

  • Lipoproteins, HDL
  • Peptides
  • Phospholipids
  • Proto-Oncogene Proteins c-bcl-2
  • RNA, Small Interfering