Elongation factor G is a critical target during oxidative damage to the translation system of Escherichia coli

J Biol Chem. 2012 Aug 17;287(34):28697-704. doi: 10.1074/jbc.M112.378067. Epub 2012 Jul 6.

Abstract

Elongation factor G (EF-G), a key protein in translational elongation, is known to be particularly susceptible to oxidation in Escherichia coli. However, neither the mechanism of the oxidation of EF-G nor the influence of its oxidation on translation is fully understood. In the present study, we investigated the effects of oxidants on the chemical properties and function of EF-G using a translation system in vitro derived from E. coli. Treatment of EF-G with 0.5 mM H(2)O(2) resulted in the complete loss of translational activity. The inactivation of EF-G by H(2)O(2) was attributable to the oxidation of two specific cysteine residues, namely, Cys(114) and Cys(266), and subsequent formation of an intramolecular disulfide bond. Replacement of Cys(114) by serine rendered EF-G insensitive to oxidation and inactivation by H(2)O(2). Furthermore, generation of the translation system in vitro with the mutated EF-G protected the entire translation system from oxidation, suggesting that EF-G might be a primary target of oxidation within the translation system. Oxidized EF-G was reactivated via reduction of the disulfide bond by thioredoxin, a ubiquitous protein that mediates dithiol-disulfide exchange. Our observations indicate that the translational machinery in E. coli is regulated, in part, by the redox state of EF-G, which might depend on the balance between the supply of reducing power and the degree of oxidative stress.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cysteine / genetics
  • Cysteine / metabolism
  • Disulfides / metabolism
  • Escherichia coli / genetics
  • Escherichia coli / metabolism*
  • Escherichia coli Proteins / genetics
  • Escherichia coli Proteins / metabolism*
  • Hydrogen Peroxide / pharmacology
  • Oxidants / pharmacology
  • Oxidation-Reduction / drug effects
  • Oxidative Stress / drug effects
  • Oxidative Stress / physiology*
  • Peptide Elongation Factor G / genetics
  • Peptide Elongation Factor G / metabolism*
  • Protein Biosynthesis / drug effects
  • Protein Biosynthesis / physiology*

Substances

  • Disulfides
  • Escherichia coli Proteins
  • Oxidants
  • Peptide Elongation Factor G
  • Hydrogen Peroxide
  • Cysteine