Targeted delivery of a combination therapy consisting of combretastatin A4 and low-dose doxorubicin against tumor neovasculature

Nanomedicine. 2012 Jan;8(1):81-92. doi: 10.1016/j.nano.2011.05.003. Epub 2011 May 20.

Abstract

The present study demonstrates the applicability of a novel strategy that employs targeted delivery of combined treatment against tumor neovasculature. Briefly, a ligand of integrins, cyclic arginine-glycine-aspartic acid-tyrosine-lysine pentapeptide (cRGDyK), was conjugated to the PEG end of polyethylene glycol-b-poly lactic acid (PEG-b-PLA), and doxorubicin was chemically linked to the PLA end of PEG-b-PLA. The targeted dual-drug micelle system was prepared by mixing combretastatin A4 (an antivascular agent), PEG-b-PLA, and the above two conjugates using a solution-casting method. The targeted micelles significantly enhanced cellular uptake of the drug by B16-F10 cells and human umbilical vein endothelial cells through a receptor-mediated endocytosis. The cRGDyK-modified dual-drug system achieved an optimal antitumor effect, lifespan increase, antineovasculature, antiproliferation, and apoptosis induction, revealing the advantage of active targeting and the modified combination therapy. In conclusion, the integration of targeted delivery and combination therapy against tumor neovasculature represents a promising approach for cancer treatment.

From the clinical editor: A ligand of integrins was conjugated to PEG-b-PLA, and doxorubicin was chemically linked to the PLA. Efficiency was demonstrated in a cancer model. The integration of targeted delivery and combination therapy against tumor neovasculature represents a promising approach for cancer treatment.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Antibiotics, Antineoplastic / administration & dosage*
  • Antibiotics, Antineoplastic / chemistry
  • Antibiotics, Antineoplastic / therapeutic use
  • Antineoplastic Agents, Phytogenic / administration & dosage*
  • Antineoplastic Agents, Phytogenic / chemistry
  • Antineoplastic Agents, Phytogenic / therapeutic use
  • Antineoplastic Combined Chemotherapy Protocols / administration & dosage*
  • Antineoplastic Combined Chemotherapy Protocols / chemistry
  • Antineoplastic Combined Chemotherapy Protocols / therapeutic use
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • Doxorubicin / administration & dosage*
  • Doxorubicin / chemistry
  • Doxorubicin / therapeutic use
  • Drug Carriers / chemistry*
  • Drug Delivery Systems
  • Human Umbilical Vein Endothelial Cells
  • Humans
  • Lactates / chemistry*
  • Lactates / therapeutic use
  • Melanoma, Experimental
  • Mice
  • Mice, Inbred C57BL
  • Micelles
  • Neovascularization, Pathologic / drug therapy
  • Peptides, Cyclic / chemistry
  • Peptides, Cyclic / therapeutic use
  • Polyethylene Glycols / chemistry*
  • Polyethylene Glycols / therapeutic use
  • Stilbenes / administration & dosage*
  • Stilbenes / chemistry
  • Stilbenes / therapeutic use

Substances

  • Antibiotics, Antineoplastic
  • Antineoplastic Agents, Phytogenic
  • Drug Carriers
  • Lactates
  • Micelles
  • Peptides, Cyclic
  • Stilbenes
  • cyclo(Arg-Gly-Asp-Tyr-Lys)
  • poly(lactic acid-ethylene glycol)
  • Polyethylene Glycols
  • Doxorubicin
  • fosbretabulin