Design, synthesis and evaluation of β-lactam antigenic peptide hybrids; unusual opening of the β-lactam ring in acidic media

Org Biomol Chem. 2010 Dec 7;8(23):5345-53. doi: 10.1039/c003877f. Epub 2010 Oct 7.

Abstract

β-Lactam peptides were envisioned as conformational constraints in antigenic peptides (APs). Three different β-lactam tripeptides of varying flexibility were prepared in solution and incorporated in place of the central part of the altered melanoma associated antigenic peptide Leu(27)-Melan-A(26-35) using solid phase synthesis techniques. Upon TFA cleavage from the solid support, an unexpected opening of the β-lactam ring occurred with conservation of the amide bond. After adaptation of the solid phase synthesis strategy, β-lactam peptides were successfully obtained and both opened and closed forms were evaluated for their capacity to bind to the antigen-presenting class-I MHC HLA-A2 protein system. None of the closed β-lactam peptides bound to HLA-A2, but their opened variants were shown to be moderate to good HLA-A2 ligands, one of them being even capable of stimulating a Melan-A-specific T cell line.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acids / chemistry*
  • Animals
  • Cells, Cultured
  • Crystallography, X-Ray
  • HLA-A2 Antigen / chemistry*
  • HLA-A2 Antigen / immunology
  • Mice
  • Models, Molecular
  • Molecular Structure
  • Peptides / chemical synthesis*
  • Peptides / immunology
  • T-Lymphocytes / immunology
  • beta-Lactams / chemistry*

Substances

  • Acids
  • HLA-A2 Antigen
  • Peptides
  • beta-Lactams