In situ DRIFTS study of hygroscopic behavior of mineral aerosol

J Environ Sci (China). 2010;22(4):555-60. doi: 10.1016/s1001-0742(09)60145-5.

Abstract

In situ diffusion reflectance infrared Fourier transform spectroscopy was used to study the water adsorption on mineral oxides (SiO2, alpha-Al2O3, MgO, Fe2O3, TiO2). The results showed that all the water adsorption isotherms were well fitted with the Brunauer-Emmett-Teller (BET)-III type equation, with the calculated monolayers occurring at 24%-30% relative humidity. It showed that about 1-5 layers of water adsorbed on oxides surfaces in ambient relative humidity (20%-90%). The measured deliquescence relative humidity of NaCl was (74 +/- 1)%, which demonstrated that DRIFTS is a useful method for the study the hygroscopic behavior of mineral dust. In addition, the limits of DRIFTS were also discussed.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adsorption
  • Aerosols
  • Air Pollutants / chemistry
  • Minerals / chemistry*
  • Oxides / chemistry
  • Spectroscopy, Fourier Transform Infrared / methods*
  • Water / chemistry*

Substances

  • Aerosols
  • Air Pollutants
  • Minerals
  • Oxides
  • Water