p47phox molecular activation for assembly of the neutrophil NADPH oxidase complex

J Biol Chem. 2010 Sep 10;285(37):28980-90. doi: 10.1074/jbc.M110.139824. Epub 2010 Jun 30.

Abstract

The p47(phox) cytosolic factor from neutrophilic NADPH oxidase has always been resistant to crystallogenesis trials due to its modular organization leading to relative flexibility. Hydrogen/deuterium exchange coupled to mass spectrometry was used to obtain structural information on the conformational mechanism that underlies p47(phox) activation. We confirmed a relative opening of the protein with exposure of the SH3 Src loops that are known to bind p22(phox) upon activation. A new surface was shown to be unmasked after activation, representing a potential autoinhibitory surface that may block the interaction of the PX domain with the membrane in the resting state. Within this surface, we identified 2 residues involved in the interaction with the PX domain. The double mutant R162A/D166A showed a higher affinity for specific phospholipids but none for the C-terminal part of p22(phox), reflecting an intermediate conformation between the autoinhibited and activated forms.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Substitution
  • Animals
  • Enzyme Activation / physiology
  • Humans
  • Mutation, Missense
  • NADPH Oxidases / chemistry*
  • NADPH Oxidases / genetics
  • NADPH Oxidases / metabolism
  • Neutrophils / enzymology*
  • Protein Structure, Secondary
  • src Homology Domains

Substances

  • NADPH Oxidases
  • CYBA protein, human
  • neutrophil cytosolic factor 1