Liquid chromatography-tandem mass spectrometry determination of oxalate in spot urine

Scand J Clin Lab Invest. 2010 Apr 19;70(3):145-50. doi: 10.3109/00365510903578765.

Abstract

Background: For assessment of total oxalic acid (OX) status, reliable quantification of OX in both urine and plasma is important. For urine, but not plasma, a commercial kit is available. We have recently described a LC-MSMS method for OX in plasma. The aim of the present study was to evaluate the usefulness of this assay for urine. We also wanted to evaluate if 24 h urine collection could be substituted by OX/creatinine-ratio (U-OX/crea) in spot-urine, and establish precursory reference intervals for U-OX/crea in children and adults.

Methods: Acidified urines were analysed and relevant validation parameters assessed. Diurnal excretion patterns were investigated in nine healthy volunteers on self-chosen diets. For method comparison, 29 urine samples were analysed with both the present method and a commercial urine-oxalate kit. Precursory reference values for U-OX/crea in children and adults (N=103, 1 month-76 years) were calculated.

Results: The within-batch coefficient of variation (CV) was 2.5% and a relative recovery of 97% in urine spiked with 5-200 micromol/L OX was found. The LC-MSMS method gave 7.9% higher OX values compared to the kit. No significant diurnal pattern of U-OX/crea was observed. U-OX/crea in children decreases with age, with no gender dependency. In adults no age variation was found, but females had somewhat higher U-OX/Crea compared to males.

Conclusion: The LC-MSMS method has proven useful for urinary OX quantification. Random spot-urine samples can be used. Age-dependent reference limits for U-OX/crea must be applied in children, in contrast to adults.

MeSH terms

  • Adult
  • Age Distribution
  • Aged
  • Aging / urine
  • Chromatography, Liquid / methods*
  • Circadian Rhythm
  • Creatinine / urine
  • Female
  • Health
  • Humans
  • Male
  • Middle Aged
  • Oxalates / urine*
  • Reference Standards
  • Reproducibility of Results
  • Tandem Mass Spectrometry / methods*

Substances

  • Oxalates
  • Creatinine