c-Jun-NH2-kinase-1 inhibition leads to antitumor activity in ovarian cancer

Clin Cancer Res. 2010 Jan 1;16(1):184-94. doi: 10.1158/1078-0432.CCR-09-1180. Epub 2009 Dec 22.

Abstract

Purpose: To show the functional, clinical, and biological significance of c-Jun-NH(2)-kinase (JNK)-1 in ovarian carcinoma.

Experimental design: Analysis of the impact of JNK on 116 epithelial ovarian cancers was conducted. The role of JNK in vitro and in experimental models of ovarian cancer was assessed. We studied the role of N-5-[4-(4-methyl piperazine methyl)-benzoylamido]-2-methylphenyl-4-[3-(4-methyl)-pyridyl]-2-pyrimidine amine (WBZ_4), a novel JNK inhibitor redesigned from imatinib based on targeting wrapping defects, in cell lines and in experimental models of ovarian cancer.

Results: We found a significant association of pJNK with progression-free survival in the 116 epithelial ovarian cancers obtained at primary debulking therapy. WBZ_4 led to cell growth inhibition and increased apoptosis in a dose-dependent fashion in four ovarian cancer cell lines. In vivo, whereas imatinib had no effect on tumor growth, WBZ_4 inhibited tumor growth in orthotopic murine models of ovarian cancer. The antitumor effect was further increased in combination with docetaxel. Silencing of JNK-1 with systemically administered siRNA led to significantly reduced tumor weights compared with nonsilencing siRNA controls, indicating that indeed the antitumor effects observed were due to JNK-1 inhibition.

Conclusions: These studies identify JNK-1 as an attractive therapeutic target in ovarian carcinoma and that the redesigned WBZ_4 compound should be considered for further clinical development.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adult
  • Aged
  • Aged, 80 and over
  • Angiogenesis Inducing Agents
  • Animals
  • Apoptosis / drug effects
  • Cell Proliferation / drug effects
  • Drug Delivery Systems
  • Enzyme Inhibitors / pharmacology
  • Female
  • Humans
  • Mice
  • Mice, Nude
  • Middle Aged
  • Mitogen-Activated Protein Kinase 8 / antagonists & inhibitors*
  • Mitogen-Activated Protein Kinase 8 / physiology*
  • Neovascularization, Pathologic / drug therapy
  • Ovarian Neoplasms / drug therapy*
  • Ovarian Neoplasms / enzymology*
  • Piperazines / pharmacology*
  • Pyrimidines / pharmacology*
  • RNA, Small Interfering / pharmacology

Substances

  • Angiogenesis Inducing Agents
  • Enzyme Inhibitors
  • N-5-(4-(4-methylpiperazinemethyl)benzoylamido)-2-methylphenyl-4-(3-(4-methyl)pyridyl)-2-pyrimidineamine
  • Piperazines
  • Pyrimidines
  • RNA, Small Interfering
  • Mitogen-Activated Protein Kinase 8