Acetyl-CoA carboxylase-alpha inhibitor TOFA induces human cancer cell apoptosis

Biochem Biophys Res Commun. 2009 Jul 31;385(3):302-6. doi: 10.1016/j.bbrc.2009.05.045. Epub 2009 May 18.

Abstract

Acetyl-CoA carboxylase-alpha (ACCA) is a rate-limiting enzyme in long chain fatty acid synthesis, playing a critical role in cellular energy storage and lipid synthesis. ACCA is upregulated in multiple types of human cancers and small interfering RNA-mediated ACCA silencing in human breast and prostate cancer cells results in oxidative stress and apoptosis. This study reports for the first time that TOFA (5-tetradecyloxy-2-furoic acid), an allosteric inhibitor of ACCA, is cytotoxic to lung cancer cells NCI-H460 and colon carcinoma cells HCT-8 and HCT-15, with an IC(50) at approximately 5.0, 5.0, and 4.5 microg/ml, respectively. TOFA at 1.0-20.0 microg/ml effectively blocked fatty acid synthesis and induced cell death in a dose-dependent manner. The cell death was characterized with PARP cleavage, DNA fragmentation, and annexin-V staining, all of which are the features of the apoptosis. Supplementing simultaneously the cells with palmitic acids (100 microM), the end-products of the fatty acid synthesis pathway, prevented the apoptosis induced by TOFA. Taken together, these data suggest that TOFA is a potent cytotoxic agent to lung and colon cancer cells, inducing apoptosis through disturbing their fatty acid synthesis.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetyl-CoA Carboxylase / antagonists & inhibitors*
  • Apoptosis* / drug effects
  • Cytotoxins / pharmacology*
  • Enzyme Inhibitors / pharmacology*
  • Furans / pharmacology*
  • Humans
  • Neoplasms / enzymology*
  • Neoplasms / pathology
  • Palmitic Acid / pharmacology

Substances

  • Cytotoxins
  • Enzyme Inhibitors
  • Furans
  • Palmitic Acid
  • 5-(tetradecyloxy)-2-furancarboxylic acid
  • Acetyl-CoA Carboxylase