Chebulinic acid and tellimagrandin I inhibit DNA strand breaks by hydroquinone/Cu(II) and H(2)O(2)/Cu(II), but potentiate DNA strand breaks by H(2)O(2)/Fe(II)

Toxicol In Vitro. 2009 Jun;23(4):667-73. doi: 10.1016/j.tiv.2009.03.009. Epub 2009 Mar 27.

Abstract

The effects of two polyphenols, chebulinic acid and tellimagrandin I, on DNA strand breaks mediated by H(2)O(2)/Cu(II), hydroquinone (HQ)/Cu(II) and H(2)O(2)/Fe(II) in pBR322 plasmid DNA and genomic DNA of cultured MRC-5 human embryo lung fibroblasts were examined. The results demonstrated that chebulinic acid and tellimagrandin I obviously inhibited HQ/Cu(II)- and H(2)O(2)/Cu(II)-mediated pBR322 DNA strand breaks. When MRC-5 cells were treated with HQ/Cu(II), the presence of chebulinic acid or tellimagrandin I inhibited HQ/Cu(II)-mediated double strand breaks of genomic DNA. The presence of chebulinic acid or tellimagrandin I did not affect the H(2)O(2)- and HQ-mediated reduction of Cu(II) to Cu(I). Both polyphenols could slightly inhibit H(2)O(2)/Fe(II)-mediated plasmid DNA strand break at the lower concentration (1-10 microM), but potentiate the DNA strand break at the higher concentration (over 50 microM). These results demonstrated that chebulinic acid and tellimagrandin I possessed antioxidant action in certain conditions and exerted prooxidant action on DNA strand breaks in other conditions.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antioxidants / pharmacology
  • Cells, Cultured
  • Copper / metabolism
  • DNA Breaks / drug effects*
  • Dose-Response Relationship, Drug
  • Gallic Acid / analogs & derivatives*
  • Gallic Acid / pharmacology
  • Glucosides / pharmacology*
  • Humans
  • Hydrogen Peroxide / toxicity*
  • Hydrolyzable Tannins / pharmacology*
  • Hydroquinones / toxicity*
  • Iron / metabolism

Substances

  • Antioxidants
  • Glucosides
  • Hydrolyzable Tannins
  • Hydroquinones
  • chebulinic acid
  • Gallic Acid
  • Copper
  • tellimagrandin I
  • Hydrogen Peroxide
  • Iron
  • hydroquinone