Synthesis and evaluation of cis-3,4-disubstituted piperidines as potent CC chemokine receptor 2 (CCR2) antagonists

Bioorg Med Chem Lett. 2008 Sep 15;18(18):5063-5. doi: 10.1016/j.bmcl.2008.07.123. Epub 2008 Aug 5.

Abstract

A series of cis-3,4-disubstituted piperidines was synthesized and evaluated as CC chemokine receptor 2 (CCR2) antagonists. Compound 24 emerged with an attractive profile, possessing excellent binding (CCR2 IC(50)=3.4 nM) and functional antagonism (calcium flux IC(50)=2.0 nM and chemotaxis IC(50)=5.4 nM). Studies to explore the binding of these piperidine analogs utilized a key CCR2 receptor mutant (E291A) with compound 14 and revealed a significant reliance on Glu291 for binding.

MeSH terms

  • Combinatorial Chemistry Techniques
  • Glutamic Acid / chemistry
  • Glutamic Acid / metabolism*
  • Inhibitory Concentration 50
  • Molecular Structure
  • Piperidines / chemical synthesis*
  • Piperidines / chemistry
  • Piperidines / pharmacology*
  • Receptors, CCR2 / antagonists & inhibitors*
  • Receptors, CCR2 / genetics
  • Stereoisomerism
  • Structure-Activity Relationship

Substances

  • Piperidines
  • Receptors, CCR2
  • Glutamic Acid