1,4-benzodiazepines as inhibitors of respiratory syncytial virus. The identification of a clinical candidate

J Med Chem. 2007 Apr 5;50(7):1685-92. doi: 10.1021/jm060747l. Epub 2007 Mar 7.

Abstract

Respiratory syncytial virus (RSV) is the cause of one-fifth of all lower respiratory tract infections worldwide and is increasingly being recognized as representing a serious threat to patient groups with poorly functioning or immature immune systems. Racemic 1,4-benzodiazepines show potent anti-RSV activity in vitro. Anti-RSV evaluation of 3-position R- and S-benzodiazepine enantiomers and subsequent optimization of this series resulted in selection of a clinical candidate. Antiviral activity was found to reside mainly in the S-enantiomer, and the R-enantiomers were consistently less active against RSV. Analogues of 1,4-(S)-benzodiazepine were synthesized as part of the lead optimization program at Arrow and tested in the XTT assay. From this exercise, (S)-1-(2-fluorophenyl)-3-(2-oxo-5-phenyl-2,3-dihydro-1H-benzo[e][1,4]-diazepin-3-yl)-urea, 17b (RSV-604) was identified as a clinical candidate, exhibiting potent anti-RSV activity in the XTT assay, which was confirmed in secondary assays. Compound 17b also possessed a good pharmacokinetic profile and has now progressed into the clinic.

MeSH terms

  • Animals
  • Antiviral Agents / chemical synthesis*
  • Antiviral Agents / pharmacokinetics
  • Antiviral Agents / pharmacology
  • Benzodiazepines / chemical synthesis*
  • Benzodiazepines / pharmacokinetics
  • Benzodiazepines / pharmacology
  • Benzodiazepinones / chemical synthesis*
  • Benzodiazepinones / pharmacokinetics
  • Benzodiazepinones / pharmacology
  • Cell Line, Tumor
  • Crystallography, X-Ray
  • Dogs
  • Enzyme-Linked Immunosorbent Assay
  • Humans
  • In Vitro Techniques
  • Microsomes / metabolism
  • Molecular Structure
  • Phenylurea Compounds / chemical synthesis*
  • Phenylurea Compounds / pharmacokinetics
  • Phenylurea Compounds / pharmacology
  • Rats
  • Respiratory Syncytial Viruses / drug effects*
  • Stereoisomerism
  • Structure-Activity Relationship
  • Viral Plaque Assay

Substances

  • 1-(2-fluorophenyl)-3-(2-oxo-5-phenyl-2,3-dihydro-1H-benzo(e)(1,4)diazepin-3-yl)urea
  • Antiviral Agents
  • Benzodiazepinones
  • Phenylurea Compounds
  • Benzodiazepines