Antileukemia activity of MSFTZ-a novel flavanone analog

Anticancer Drugs. 2006 Jul;17(6):641-7. doi: 10.1097/01.cad.0000215060.70566.59.

Abstract

A newly synthesized flavanone derivative, (+/-)-(3aRS,4SR)-2-(2-chloro-4-methyl- sulfonylphenyl)-4'-chloro-3a,4-diethoxy-flavane[4,3-d]-Delta-1,2,3-thiadiazoline (MSFTZ), was investigated for its antileukemia activity and molecular mechanisms. Cytotoxicity assay confirmed the high antiproliferative efficiency of MSFTZ in six leukemia cell lines (including two drug-resistant cell lines), with 50% inhibition of cell viability values ranging from 1.0 to 9.2 micromol/l. The results of flow cytometry assay showed that the percentage of apoptotic HL-60 cells was 68.3% after 48 h treatment with MSFTZ, suggesting that the activation of the apoptosis pathway was an anticancer property of MSFTZ. Furthermore, the protein changes related to apoptosis were investigated. Exposure of HL-60 cells to MSFTZ induced pro-caspase-9 and pro-caspase-3 cleavage, X-linked inhibitor of apoptosis protein and Bcl-X(L) downregulation, and poly(ADP-ribose) polymerase degradation. Treatment of cells with MSFTZ resulted in a time-dependent reduction in phosphorylation (activation) of extracellular signal-regulated kinase 1/2 and an increase in phosphorylation (activation) of Jun N-terminal kinase. Taken together, our results demonstrated that activation of mitogen-activated protein kinase and apoptotic cascade is involved in MSFTZ-induced antileukemia activity. All data suggest that MSFTZ is a promising chemotherapy drug.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antineoplastic Agents / therapeutic use*
  • Apoptosis / drug effects
  • Benzopyrans / chemistry
  • Benzopyrans / therapeutic use*
  • Blotting, Western
  • Caspase 3 / metabolism
  • Caspase 9 / metabolism
  • Cell Proliferation / drug effects
  • Enzyme Activation / drug effects
  • Flavanones / therapeutic use*
  • Flow Cytometry
  • HL-60 Cells
  • Humans
  • JNK Mitogen-Activated Protein Kinases / metabolism
  • Leukemia / drug therapy*
  • Leukemia / metabolism
  • Mitogen-Activated Protein Kinase 1 / metabolism
  • Mitogen-Activated Protein Kinase 3 / metabolism
  • Phosphorylation / drug effects
  • Poly(ADP-ribose) Polymerases / metabolism
  • Proto-Oncogene Proteins c-bcl-2 / metabolism
  • Thiadiazoles / chemistry
  • Thiadiazoles / therapeutic use*
  • Tumor Cells, Cultured

Substances

  • 2-(2-chloro-4-methylsulfonylphenyl)-4'-chloro-3a,4-diethoxyflavane(4,3-d)-delta(1,9b)-1,2,3-thiadiazoline
  • Antineoplastic Agents
  • Benzopyrans
  • Flavanones
  • Proto-Oncogene Proteins c-bcl-2
  • Thiadiazoles
  • Poly(ADP-ribose) Polymerases
  • JNK Mitogen-Activated Protein Kinases
  • Mitogen-Activated Protein Kinase 1
  • Mitogen-Activated Protein Kinase 3
  • Caspase 3
  • Caspase 9