Photoelectron spectroscopy on thin films of extended zinc porphyrazines

J Phys Chem B. 2005 Apr 28;109(16):7826-33. doi: 10.1021/jp046576i.

Abstract

Photoemission measurements were performed on a series of stepwise benzoannelated zinc porphyrazine molecules in thin films. The electronic structure of tert-butyl-substituted zinc tetraazaporphyrin, phthalocyanine, and naphthalocyanine is investigated using mainly EUV synchrotron radiation. A detailed analysis of the zinc satellites in the spectra of the valence region is performed in an attempt to infer the effect of ligand size extension on the metal-ligand interactions. No differences in the character of the bond between zinc and ligand were detected as a function of ligand size. The results are compared with those for the respective metal-free and copper-containing molecules.

MeSH terms

  • Organometallic Compounds / chemistry*
  • Spectrophotometry
  • Zinc / chemistry*

Substances

  • Organometallic Compounds
  • Zinc