A new class of inhibitors of 2-arachidonoylglycerol hydrolysis and invasion of prostate cancer cells

Biochem Biophys Res Commun. 2005 Jul 15;332(4):1028-33. doi: 10.1016/j.bbrc.2005.05.049.

Abstract

Endogenous 2-arachidonoylglycerol (2-AG) inhibits invasion of androgen-independent prostate cancer cells. Blocking cellular hydrolysis of 2-AG to increase its endogenous concentration results in a decrease in cell invasion. A series of compounds containing a trifluoromethyl ketone (TFK) moiety or the methyl analog (known to inhibit carboxylesterases) were investigated for their ability to inhibit 2-AG hydrolysis and prostate cancer cell invasion. Compounds containing a thioether beta to a TFK moiety inhibited 2-AG hydrolysis as well as cell invasion in a concentration-dependent manner. Inhibition of 2-AG hydrolysis increased concomitantly with inhibitor alkyl chain length from 4- to 12-carbons while inhibition of cell invasion exhibited a maximum at 8- to 10-carbons of the compounds. These results demonstrate a new series of 2-AG hydrolysis inhibitors as a potential therapeutic approach for prostate cancer.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Antineoplastic Agents / pharmacology*
  • Arachidonic Acids / metabolism*
  • Cannabinoid Receptor Modulators / metabolism
  • Cell Line, Tumor
  • Chromatography, Liquid
  • Collagen / chemistry
  • Dose-Response Relationship, Drug
  • Drug Combinations
  • Endocannabinoids
  • Enzyme Inhibitors / pharmacology*
  • Glycerides / metabolism*
  • Humans
  • Hydrolysis
  • Ketones / chemistry
  • Laminin / chemistry
  • Male
  • Models, Chemical
  • Neoplasm Invasiveness
  • Prostatic Neoplasms / pathology*
  • Proteoglycans / chemistry
  • Spectrometry, Mass, Electrospray Ionization
  • Sulfides / chemistry

Substances

  • Antineoplastic Agents
  • Arachidonic Acids
  • Cannabinoid Receptor Modulators
  • Drug Combinations
  • Endocannabinoids
  • Enzyme Inhibitors
  • Glycerides
  • Ketones
  • Laminin
  • Proteoglycans
  • Sulfides
  • matrigel
  • glyceryl 2-arachidonate
  • Collagen