Hydrolysis of bimatoprost (Lumigan) to its free acid by ocular tissue in vitro

J Ocul Pharmacol Ther. 2003 Feb;19(1):45-54. doi: 10.1089/108076803762718105.

Abstract

We determined whether bimatoprost, which has been reported to act via putative prostamide receptors, could be hydrolyzed to its free acid (17-phenyl-PGF(2 alpha)), a potent FP receptor agonist, by human ocular tissue in vitro. We developed a gas chromatography/mass spectrometric method to measure 17-phenyl-PGF(2 alpha) levels at sub-picomolar levels. We then analyzed the amount of 17-phenyl-PGF(2 alpha) present after incubation of 50 microl Lumigan (0.03% bimatoprost) with eye tissue using this assay. We found that cornea, sclera, iris, and ciliary body, all rapidly hydrolyzed bimatoprost to 17-phenyl-PGF(2 alpha) with linear kinetics at a rate of 6.3, 2.0, 2.8, and 1.5 pmol mg tissue(-1) hr(-1), respectively. For cornea, sclera, and ciliary body, this linear rate of hydrolysis continued over a period of at least three hours, while iris-induced hydrolysis did not continue beyond one hour. Our findings suggest that bimatoprost can act as prodrug for FP receptor activation and questions the concept of a "prostamide receptor" agonist.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amides
  • Animals
  • Bimatoprost
  • Ciliary Body / metabolism
  • Cloprostenol / analogs & derivatives
  • Cornea / metabolism
  • Dinoprost / analogs & derivatives*
  • Dinoprost / biosynthesis*
  • Eye / metabolism*
  • Humans
  • Hydrolysis
  • In Vitro Techniques
  • Iris / metabolism
  • Kinetics
  • Lipid Metabolism*
  • Lipids
  • Prodrugs / metabolism*
  • Sclera / metabolism
  • Swine
  • Time Factors

Substances

  • Amides
  • Lipids
  • Prodrugs
  • Cloprostenol
  • 17-phenylprostaglandin F2alpha
  • Dinoprost
  • Bimatoprost