Purification and characterization of a thermostable alpha-galactosidase from Thermoanaerobacterium polysaccharolyticum

J Agric Food Chem. 2002 Sep 25;50(20):5676-82. doi: 10.1021/jf0202281.

Abstract

Food ingredients containing alpha-1,6-galactoside bonds elicit gastrointestinal disturbances in monogastric animals, including humans. Pretreatment of such ingredients with alpha-galactosidase (EC 3.2.1.22) has the potential to alleviate this condition. For this purpose, a thermostable alpha-galactosidase from Thermoanaerobacterium polysaccharolyticum was purified by a combination of anion exchange and size exclusion chromatographies. The enzyme has a monomeric molecular weight of approximately 80 kDa; however, it is active as a dimer. The optimum temperature for enzyme activity is 77.5 degrees C. Approximately 84 and 88% of enzyme activity remained after 36.5 h of incubation at 70 and 65 degrees C, respectively. Optimum activity was observed at pH 8.0, with a broad range of activity from pH 5.0 to 9.0. Different transition metals had weak to strong inhibitory effects on enzyme activity. The K(m) and V(max) of the enzyme are 0.29-0.345 mM and 200-232 micromol/min/mg of protein, respectively. Importantly, enzyme activity was only slightly inhibited by 75-100 mM galactose, an end product of hydrolysis. Enzyme activity was specific for the alpha-1,6-galactosyl bond, and activity was demonstrated on melibiose and soy molasses.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Clostridium / enzymology*
  • Dimerization
  • Enzyme Stability
  • Hydrogen-Ion Concentration
  • Molecular Sequence Data
  • Molecular Weight
  • alpha-Galactosidase / chemistry
  • alpha-Galactosidase / isolation & purification*
  • alpha-Galactosidase / metabolism*

Substances

  • alpha-Galactosidase