Licofelone (ML-3000), a dual inhibitor of 5-lipoxygenase and cyclooxygenase, reduces the level of cartilage chondrocyte death in vivo in experimental dog osteoarthritis: inhibition of pro-apoptotic factors

J Rheumatol. 2002 Jul;29(7):1446-53.

Abstract

Objective: To evaluate in vivo therapeutic efficacy of licofelone, a novel competitive dual inhibitor of 5-lipoxygenase (5-LOX) and cyclooxygenase (COX) in chondrocyte death in the canine ligament transection model of osteoarthritis (OA), and to explore its effect on factors involved in the apoptotic phenomenon, i.e., caspase-3, COX-2, and inducible nitric oxide synthase (iNOS).

Methods: Cartilage specimens were obtained from 3 experimental groups of dogs: Group 1, dogs subjected to sectioning of the anterior cruciate ligament of the right knee and given placebo treatment; Groups 2 and 3, operated dogs that received oral treatment with licofelone (2.5 or 5.0 mg/kg/day, respectively) for 8 weeks starting immediately after surgery. All dogs were killed 8 weeks postsurgery. The cartilage level of chondrocyte death was detected by TUNEL reaction. Cartilage distribution of caspase-3, COX-2, and iNOS was documented by immunohistochemistry using specific antibodies, and other levels were quantified by morphometric analysis.

Results: In cartilage specimens from placebo treated dogs a large number of chondrocytes in the superficial layers stained positive for TUNEL reaction. Treatment with therapeutic concentrations of licofelone (2.5 and 5.0 mg/kg/day) markedly reduced the level of chondrocyte apoptosis to the same extent in both therapeutic groups (p < 0.0001, p < 0.002, respectively). In these groups, the levels of caspase-3, COX-2, and iNOS in cartilage from both condyles and plateaus were also significantly decreased (p < 0.0001, p < 0.0001, p < 0.0002, respectively) compared to the control (placebo) group.

Conclusion: Licofelone is an effective treatment in vivo, capable of reducing the level of OA chondrocyte death. This effect is likely mediated by a decrease in the level of caspase-3 activity, which may be related to the reduced production of 2 major factors involved in chondrocyte apoptosis, NO and prostaglandin E2. These findings may explain some of the mechanisms by which licofelone reduces the progression of experimental OA.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetates / pharmacology*
  • Administration, Oral
  • Animals
  • Apoptosis / drug effects*
  • Cartilage, Articular / cytology
  • Cartilage, Articular / drug effects*
  • Chondrocytes / drug effects
  • Chondrocytes / physiology*
  • Disease Models, Animal
  • Dogs
  • Dose-Response Relationship, Drug
  • Drug Administration Schedule
  • Immunohistochemistry
  • Interleukin-1 / analysis
  • Matrix Metalloproteinase 1 / analysis
  • Nitric Oxide Synthase / drug effects
  • Nitric Oxide Synthase / metabolism
  • Osteoarthritis / drug therapy*
  • Osteoarthritis / pathology*
  • Probability
  • Pyrroles / pharmacology*
  • Reference Values
  • Sensitivity and Specificity
  • Statistics, Nonparametric

Substances

  • Acetates
  • Interleukin-1
  • Pyrroles
  • Nitric Oxide Synthase
  • Matrix Metalloproteinase 1
  • licofelone