Antibody catalysis of the oxidation of water

Science. 2001 Sep 7;293(5536):1806-11. doi: 10.1126/science.1062722.

Abstract

Recently we reported that antibodies can generate hydrogen peroxide (H2O2) from singlet molecular oxygen (1O2*). We now show that this process is catalytic, and we identify the electron source for a quasi-unlimited generation of H2O2. Antibodies produce up to 500 mole equivalents of H2O2 from 1O2*, without a reduction in rate, and we have excluded metals or Cl- as the electron source. On the basis of isotope incorporation experiments and kinetic data, we propose that antibodies use H2O as an electron source, facilitating its addition to 1O2* to form H2O3 as the first intermediate in a reaction cascade that eventually leads to H2O2. X-ray crystallographic studies with xenon point to putative conserved oxygen binding sites within the antibody fold where this chemistry could be initiated. Our findings suggest a protective function of immunoglobulins against 1O2* and raise the question of whether the need to detoxify 1O2* has played a decisive role in the evolution of the immunoglobulin fold.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Antibodies, Catalytic / chemistry
  • Antibodies, Catalytic / metabolism*
  • Binding Sites
  • Catalysis
  • Conserved Sequence
  • Crystallography, X-Ray
  • Humans
  • Hydrogen Peroxide / metabolism*
  • Kinetics
  • Models, Molecular
  • Oxidants / chemistry
  • Oxidants / metabolism*
  • Oxidation-Reduction
  • Oxygen / metabolism*
  • Protein Conformation
  • Singlet Oxygen
  • Spectrometry, Mass, Electrospray Ionization
  • Thermodynamics
  • Tryptophan / metabolism
  • Ultraviolet Rays
  • Water / chemistry*
  • Water / metabolism*
  • Xenon / metabolism

Substances

  • Antibodies, Catalytic
  • Oxidants
  • Water
  • Singlet Oxygen
  • Xenon
  • Tryptophan
  • Hydrogen Peroxide
  • Oxygen