Infrared laser spectroscopy of jet-cooled carbon clusters: structure of triplet C6

Mol Phys. 1993;79(4):769-76. doi: 10.1080/00268979300101611.

Abstract

We report the first structural characterization of the triplet isomer of C6. Forty-one rovibrational/fine structure transitions in the nu 4(sigma u) antisymmetric stretch fundamental of the C6 cluster have been measured by diode laser absorption spectroscopy of a supersonic carbon cluster beam. The observed spectrum is characteristic of a centrosymmetric linear triplet state with cumulene-type bonding. The measured ground state rotational constant B0 = 0.048 479 (10)cm-1 and the effective bond length r(eff) = 1.2868 (1) angstroms are in good agreement with ab initio predictions for the linear triplet (3 sigma g-) state of C6.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Astronomy / instrumentation
  • Astronomy / methods*
  • Carbon / chemistry*
  • Chemistry Techniques, Analytical / instrumentation
  • Chemistry Techniques, Analytical / methods
  • Molecular Structure
  • Spectrophotometry, Infrared

Substances

  • Carbon